This paper provides insights into the radioactivity levels in soil, sediment and surface seawater from selected monitoring sites in Singapore. The environmental samples were measured for naturally occurring and anthropogenic radionuclides. In soils, the decay series of 232Th and 238U are the highest contributors to the total radioactivity, while in sediments, 40K is the main contributor to the total radioactivity. The levels of 90Sr, 137Cs and 239+240Pu are also reported. The data demonstrates that the main source of anthropogenic radionuclides in soils is the global fallout from nuclear weapons testings; in sediments, contributions from the Pacific Proving Grounds have been identified. This study also highlights significant differences in radioactivity levels in soils between the northern and central regions of Singapore, which are attributed to the histories of the monitoring sites.