An inventory of aquatic and terrestrial Heteroptera (excluding Aradidae, Coreidae and Pentatomoidea), comprising 101 species in 23 families, collected in the Chaco National Park (NE Argentina) is presented. . Fifty species are new records to the Argentinean Chaco province, and six species represent new records to Argentina: Cryphula affinis (Distant), Valtissius distinctus (Distant) (Rhyparochromidae), Stenopoda subinermis Stål, Diaditus pilosicornis Bergroth (Reduviidae), Buenoa uhleri Truxal (Notonectidae), and Paravelia splendoris (Drake & Harris) (Veliidae).