The fragment mass analyzer at the ATLAS facility has been used to unambiguously identify the mass number associated with different decay modes of the nobelium isotopes produced via 204 Pb(48 Ca, xn) 252−x No reactions. Isotopically pure (>99.7%) 204 Pb targets were used to reduce background from more favored reactions on heavier lead isotopes. Two spontaneous fission half-lives (t 1/2 = 3.7 +1.1 −0.8 and 43 +22 −15 µs) were deduced from a total of 158 fission events. Both decays originate from 250 No rather than from neighboring isotopes as previously suggested. The longer activity most likely corresponds to a K isomer in this nucleus. No conclusive evidence for an α branch was observed, resulting in upper limits of 2.1% for the shorter lifetime and 3.4% for the longer activity.

Electromagnetic transition probabilities have been measured for the intraband and interband transitions in the two sequences in the nucleus (135)Nd that were previously identified as a composite chiral pair of rotational bands. The chiral character of the bands is affirmed and it is shown that their behavior is associated with a transition from a vibrational into a static chiral regime.

Excited states in 64 Ni, 66 Ni, and 68 Ni were populated in quasielastic and deep-inelastic reactions of a 430-MeV 64 Ni beam on a thick 238 U target. Level schemes including many nonyrast states were established up to respective excitation energies of 6.8, 8.2, and 7.8 MeV on the basis of γ -ray coincidence events measured with the Gammasphere array. Spin-parity assignments were deduced from an angular-correlation analysis and from observed γ -decay patterns, but information from earlier γ -spectroscopy and nuclear-reaction studies was used as well. The spin assignments for nonyrast states were supported further by their observed population pattern in quasielastic reactions selected through a cross-coincidence technique. Previously established isomeric-state decays in 66 Ni and 68 Ni were verified and delineated more extensively through a delayed-coincidence analysis. A number of new states located above these long-lived states were identified. Shell-model calculations were carried out in the p 3/2 f 5/2 p 1/2 g 9/2 model space with two effective interactions using a 56 Ni core. Satisfactory agreement between experimental and computed level energies was achieved, even though the calculations indicate that all the states are associated with rather complex configurations. This complexity is illustrated through the discussion of the structure of the negative-parity states and of the M1 decays between them. The best agreement between data and calculations was achieved for 68 Ni, the nucleus where the calculated states have the simplest structure. In this nucleus, the existence of two low-spin states reported recently was confirmed as well. Results of the present study do not indicate any involvement of collective degrees of freedom and confirm the validity of a shell-model description in terms of neutron excitations combined with a closed Z = 28 proton shell. Further improvements to the calculations are desirable.

We have identified two isomers in 254No, built on two- and four-quasiparticle excitations, with quantum numbers K pi = 8- and (14+), as well as a low-energy 2-quasiparticle Kpi = 3+ state. The occurrence of isomers establishes that K is a good quantum number and therefore that the nucleus has an axial prolate shape. The 2-quasiparticle states probe the energies of the proton levels that govern the stability of superheavy nuclei, test 2-quasiparticle energies from theory, and thereby check their predictions of magic gaps.