How the interacting electronic states and phases of layered transition-metal dichalcogenides evolve when thinned to the single-layer limit is a key open question in the study of two-dimensional materials. Here, we use angle-resolved photoemission to investigate the electronic structure of monolayer VSe grown on bilayer graphene/SiC. While the global electronic structure is similar to that of bulk VSe, we show that, for the monolayer, pronounced energy gaps develop over the entire Fermi surface with decreasing temperature below T = 140 ± 5 K, concomitant with the emergence of charge-order superstructures evident in low-energy electron diffraction. These observations point to a charge-density wave instability in the monolayer that is strongly enhanced over that of the bulk. Moreover, our measurements of both the electronic structure and of X-ray magnetic circular dichroism reveal no signatures of a ferromagnetic ordering, in contrast to the results of a recent experimental study as well as expectations from density functional theory. Our study thus points to a delicate balance that can be realized between competing interacting states and phases in monolayer transition-metal dichalcogenides.
Si nanowires grow rapidly by chemical vapor deposition on Ti-containing islands on Si surfaces when an abundant supply of Si-containing gaseous precursor is available. The density of wires is approximately the same as the density of the nucleating islands on the Si surface, although at least two different types of islands appear to correlate with very different wire growth rates. For the deposition conditions used, a minority of long, defect-free wires form, along with more numerous wires containing defects. Energy-dispersive x-ray spectroscopy shows that the Ti-containing nanoparticles remain at the tip of the growing wires. The estimated diffusion coefficient of Si in TiSi2 is consistent with the catalyzing nanoparticle remaining in the solid phase during nanowire growth.
wordsMagnetic skyrmions are topologically non-trivial nanoscale objects. Their topology, which originates in their chiral domain wall winding, governs their unique response to a motion-inducing force. When subjected to an electrical current, the chiral winding of the spin texture leads to a deflection of the skyrmion trajectory, characterized by an angle with respect to the applied force direction. This skyrmion Hall angle was believed to be skyrmion diameter-dependent. In contrast, our experimental study finds that within the plastic flow regime the skyrmion Hall angle is diameter-independent. At an average velocity of 6 ± 1 m/s the average skyrmion Hall angle was measured to be 9° ± 2°. In fact, in the plastic flow regime, the skyrmion dynamics is dominated by the local energy landscape such as materials defects and the local magnetic configuration.
Room temperature magnetic skyrmions in magnetic multilayers are considered as information carriers for future spintronic applications. Currently, a detailed understanding of the skyrmion stabilization mechanisms is still lacking in these systems. To gain more insight, it is first and foremost essential to determine the full real‐space spin configuration. Here, two advanced X‐ray techniques are applied, based on magnetic circular dichroism, to investigate the spin textures of skyrmions in [Ta/CoFeB/MgO]n multilayers. First, by using ptychography, a high‐resolution diffraction imaging technique, the 2D out‐of‐plane spin profile of skyrmions with a spatial resolution of 10 nm is determined. Second, by performing circular dichroism in resonant elastic X‐ray scattering, it is demonstrated that the chirality of the magnetic structure undergoes a depth‐dependent evolution. This suggests that the skyrmion structure is a complex 3D structure rather than an identical planar texture throughout the layer stack. The analyses of the spin textures confirm the theoretical predictions that the dipole–dipole interactions together with the external magnetic field play an important role in stabilizing sub‐100 nm diameter skyrmions and the hybrid structure of the skyrmion domain wall. This combined X‐ray‐based approach opens the door for in‐depth studies of magnetic skyrmion systems, which allows for precise engineering of optimized skyrmion heterostructures.
The combination of topological insulators, that is, bulk insulators with gapless, topologically protected surface states, with magnetic order is a love-hate relationship that can unlock new quantum states and exotic physical phenomena, such as the quantum anomalous Hall effect and axion electrodynamics. Moreover, the unusual coupling between topological insulators and ferromagnets can also result in the formation of topological spin textures in the ferromagnetic layer. Skyrmions are topologically protected magnetization swirls that are promising candidates for spintronics memory carriers. Here, we report on the observation of skyrmionium in thin ferromagnetic films coupled to a magnetic topological insulator. The occurrence of skyrmionium, which appears as a soliton composed of two skyrmions with opposite winding numbers, is tied to the ferromagnetic state of the topological insulator. Our work presents a new combination of two important classes of topological materials and may open the door to new topologically inspired information-storage concepts in the future.
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