Morpho sulkowskyi butterfly wings contain naturally occurring hierarchical nanostructures that produce structural coloration. The high aspect ratio and surface area of these wings make them attractive nanostructured templates for applications in solar energy and photocatalysis. However, biomimetic approaches to replicate their complex structural features and integrate functional materials into their three-dimensional framework are highly limited in precision and scalability. Herein, a biotemplating approach is presented that precisely replicates Morpho nanostructures by depositing nanocrystalline ZnO coatings onto wings via low-temperature atomic layer deposition (ALD). This study demonstrates the ability to precisely tune the natural structural coloration while also integrating multifunctionality by imparting photocatalytic activity onto fully intact Morpho wings. Optical spectroscopy and finite-difference time-domain numerical modeling demonstrate that ALD ZnO coatings can rationally tune the structural coloration across the visible spectrum. These structurally colored photocatalysts exhibit an optimal coating thickness to maximize photocatalytic activity, which is attributed to trade-offs between light absorption and catalytic quantum yield with increasing coating thickness. These multifunctional photocatalysts present a new approach to integrating solar energy harvesting into visually attractive surfaces that can be integrated into building facades or other macroscopic structures to impart aesthetic appeal.

Noncontact human-machine interaction provides a hygienic and intelligent approach for the communication between human and robots. Current noncontact human-machine interactions are generally limited by the interaction distance or conditions, such as in the dark. Here we explore the utilization of hand as an infrared light source for noncontact human-machine interaction. Metallic gratings are used as the human-machine interface to respond to infrared radiation from hand and the generated signals are visualized as different infrared structural colors. We demonstrate the applications of the infrared structural color-based human-machine interaction for user-interactive touchless display and real-time control of a robot vehicle. The interaction is flexible to the hand-interface distance ranging from a few centimeters to tens of centimeters and can be used in low lighting condition or in the dark. The findings in this work provide an alternative and complementary approach to traditional noncontact human-machine interactions, which may further broaden the potential applications of human-machine interaction.

Three-dimensional heterogeneous nanostructures that integrate plasmonic nanostructures of Pd with photonic architecture of Morpho butterfly wings can achieve sensitive hydrogen gas detection.

Solar-driven interfacial evaporation, as one of the most effective ways to convert and utilize solar energy, has attracted lot of interest recently. Most of the previous research studies, however, mainly focused on nonpatterned solar absorbers by improving the structural and chemical characteristics of the solar absorbers used in the interfacial evaporation systems. In this work, we investigated the influence of patterned surface on the evaporation performance of solar absorbers. The patterned surfaces studied, which include black patterns and white patterns, were achieved by selectively printing carbon black on the air-laid paper. Such a design leads to the lateral temperature differences between adjacent patterns of the solar absorber under solar illumination. The temperature differences result in the lateral heat and mass transfer between those patterns, which can effectively accelerate solar-driven vapor generation. With similar patterns and same coverage of carbon black, the increase in the circumference of the surface patterns leads to the increase in the evaporation performance. Additionally, we found that the evaporation performance can be optimized through the design of surface patterns, which demonstrates the potential in reducing the usage of the light-absorbing materials in the solar absorber. The findings in this work not only expand the understanding of the interfacial evaporation systems but also offer additional guidelines in designing interfacial evaporation systems.

Human skin shows self‐adaptive temperature regulation through both enhanced heat dissipation in high temperature environments and depressed heat dissipation in cold environments. Inspired by such thermal regulation processes, an interfacial material system with self‐adaptive temperature regulation in the solar‐driven interfacial evaporation system, which can exhibit automatic temperature oscillation to enable pyroelectricity generation while producing water vapor, is reported. The bioinspired interface system is designed with the combination of a thermochromism‐based temperature regulator consisting of tungsten‐doped vanadium dioxide nanoparticles and a polymeric pyroelectric thin film of polyvinylidene fluoride. Under the simulated solar illumination with power density of 1.1 kW m−2, the bioinspired interfacial evaporation system achieves a self‐adaptive temperature oscillation with the maximum temperature difference of ≈7 °C and this system can simultaneously generate water vapor as well as electricity with an evaporation efficiency of 71.43% and a maximum output electrical power density of 104 µW m−2, respectively. The study demonstrates a design of thermal management at the interface of solar‐driven evaporation system to exhibit a self‐adaptive temperature oscillation and offers an alternative approach for the multifunctional harvesting of solar energy.