Abstract. The global methane (CH 4 ) budget is becoming an increasingly important component for managing realistic pathways to mitigate climate change. This relevance, due to a shorter atmospheric lifetime and a stronger warming potential than carbon dioxide, is challenged by the still unexplained changes of atmospheric CH 4 over the past decade. Emissions and concentrations of CH 4 are continuing to increase, making CH 4 the second most important human-induced greenhouse gas after carbon dioxide. Two major difficulties in reducing uncertainties come from the large variety of diffusive CH 4 sources that overlap geographically, and from the destruction of CH 4 by the very short-lived hydroxyl radical (OH). To address these difficulties, we have established a consortium of multi-disciplinary scientists under the umbrella of the Global Carbon Project to synthesize and stimulate research on the methane cycle, and producing regular (∼ biennial) updates of the global methane budget. This consortium includes atmospheric physicists and chemists, biogeochemists of surface and marine emissions, and socio-economists who study anthropogenic emissions. Following Kirschke et al. (2013), we propose here the first version of a living review paper that integrates results of top-down studies (exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models, inventories and data-driven approaches (including process-based models for estimating land surface emissions and atmospheric chemistry, and inventories for anthropogenic emissions, data-driven extrapolations). . Top-down inversions consistently infer lower emissions in China (∼ 58 Tg CH 4 yr −1 , range 51-72, −14 %) and higher emissions in Africa (86 Tg CH 4 yr −1 , range 73-108, +19 %) than bottom-up values used as prior estimates. Overall, uncertainties for anthropogenic emissions appear smaller than those from natural sources, and the uncertainties on source categories appear larger for top-down inversions than for bottom-up inventories and models.The most important source of uncertainty on the methane budget is attributable to emissions from wetland and other inland waters. We show that the wetland extent could contribute 30-40 % on the estimated range for wetland emissions. Other priorities for improving the methane budget include the following: (i) the development of process-based models for inland-water emissions, (ii) the intensification of methane observations at local scale (flux measurements) to constrain bottom-up land surface models, and at regional scale (surface networks and satellites) to constrain top-down inversions, (iii) improvements in the estimation of atmospheric loss by OH, and (iv) improvements of the transport models integrated in top-down inversions.
Abstract. Wetland emissions remain one of the principal sources of uncertainty in the global atmospheric methane (CH 4 ) budget, largely due to poorly constrained process controls on CH 4 production in waterlogged soils. Process-based estimates of global wetland CH 4 emissions and their associated uncertainties can provide crucial prior information for model-based top-down CH 4 emission estimates. Here we construct a global wetland CH 4 emission model ensemble for use in atmospheric chemical transport models (WetCHARTs version 1.0). Our 0.5 • × 0.5 • resolution model ensemble is based on satellite-derived surface water extent and precipitation reanalyses, nine heterotrophic respiration simulations (eight carbon cycle models and a data-constrained terrestrial carbon cycle analysis) and three temperature dependence parameterizations for the period 2009-2010; an extended ensemble subset based solely on precipitation and the data-constrained terrestrial carbon cycle analysis is derived for the period 2001-2015. We incorporate the mean of the full and extended model ensembles into GEOS-Chem and compare the model against surface measurements of atmospheric CH 4 ; the model performance (site-level and zonal mean anomaly residuals) compares favourably against published wetland CH 4 emissions scenarios. We find that uncertainties in carbon decomposition rates and the wetland extent together account for more than 80 % of the dominant uncertainty in the timing, magnitude and seasonal variability in wetland CH 4 emissions, although uncertainty in the temperature CH 4 : C dependence is a significant contributor to seasonal variations in mid-latitude wetland CH 4 emissions. The combination of satellite, carbon cycle models and temperature dependence parameterizations provides a physically informed structural a priori uncertainty that is critical for topdown estimates of wetland CH 4 fluxes. Specifically, our ensemble can provide enhanced information on the prior CH 4 emission uncertainty and the error covariance structure, as well as a means for using posterior flux estimates and their uncertainties to quantitatively constrain the biogeochemical process controls of global wetland CH 4 emissions.
Increasing atmospheric methane (CH 4 ) concentrations have contributed to approximately 20% of anthropogenic climate change. Despite the importance of CH 4 as a greenhouse gas, its atmospheric growth rate and dynamics over the past two decades, which include a stabilization period (1999)(2000)(2001)(2002)(2003)(2004)(2005)(2006), followed by renewed growth starting in 2007, remain poorly understood. We provide an updated estimate of CH 4 emissions from wetlands, the largest natural global CH 4 source, for 2000-2012 using an ensemble of biogeochemical models constrained with remote sensing surface inundation and inventory-based wetland area data. Between 2000-2012, boreal wetland CH 4 emissions increased by 1.2 Tg yr −1 (−0.2-3.5 Tg yr −1 ), tropical emissions decreased by 0.9 Tg yr −1 (−3.2−1.1 Tg yr −1 ), yet globally, emissions remained unchanged at 184 ± 22 Tg yr −1 . Changing air temperature was responsible for increasing high-latitude emissions whereas declines in low-latitude wetland area decreased tropical emissions; both dynamics are consistent with features of predicted centennial-scale climate change impacts on wetland CH 4 emissions. Despite uncertainties in wetland area mapping, our study shows that global wetland CH 4 emissions have not contributed significantly to the period of renewed atmospheric CH 4 growth, and is consistent with findings from studies that indicate some combination of increasing fossil fuel and agriculture-related CH 4 emissions, and a decrease in the atmospheric oxidative sink.
Abstract. Following the recent Global Carbon Project (GCP) synthesis of the decadal methane (CH 4 ) budget over 2000, we analyse here the same dataset with a focus on quasi-decadal and inter-annual variability in CH 4 emissions. The GCP dataset integrates results from topdown studies (exploiting atmospheric observations within an atmospheric inverse-modelling framework) and bottom-up models (including process-based models for estimating land surface emissions and atmospheric chemistry), inventories of anthropogenic emissions, and data-driven approaches.The annual global methane emissions from top-down studies, which by construction match the observed methane growth rate within their uncertainties, all show an increase in total methane emissions over the period [2000][2001][2002][2003][2004][2005][2006][2007][2008][2009][2010][2011][2012], but this increase is not linear over the 13 years. Despite differences between individual studies, the mean emission anomaly of
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
hi@scite.ai
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.