Herein, we report the performance of CsPbX (X = Cl, Br, and I) perovskite quantum dots (QDs) for photocatalytic degradation of organic dyes. The photocatalytic performance of CsPbX QDs was characterized by UV-vis absorption spectra and ESI-MS, which evaluated their ability of degrading methyl orange (MO) solution under visible light irradiation. Interestingly, both CsPbCl and CsPbBr QDs show excellent photocatalytic activities, which can decompose the MO solution into a colorless solution within 100 min. This study demonstrates the potential of CsPbX QDs in the degradation of organic dyes and environmentally friendly applications. Moreover, the integration of CsPbX QDs and photocatalysis provides a new insight for the design of new photocatalysts.
We propose and experimentally demonstrate a high efficient circularly polarizing dichroism waveplate (CPDW) using a Si-based all-dielectric 2Dchiral metasurface. We demonstrate that the CPDW exhibits a unique dichroism in that it functions as a transmissive quarter waveplate for one of either left-or right-handed circularly polarized incident lightand a reflective mirror for the opposite polarization. The circular polarization dichroism (CPD = IRCP − ILCP) in transmission at wavelength ~1.5 μm reaches 97% and the extinction ratio (ER = IRCP/ILCP) is as high as 345:1. Experimental fabrications and measurements of the proposed all-dielectric metasurface are implemented and found to be in excellent agreement with the simulations. The proposed all-dielectric chiral metasurface is of advantages of high-dichroism, easy-fabrication and standard semiconductor fabrication techniques compatible, which could lead to enhanced security in fiber and free-space communications, as well as imaging and sensing applications for circularly polarized light with a highly integrated photonic platform.
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