Today's most precise time and frequency measurements are performed with optical atomic clocks. However, it has been proposed that they could potentially be outperformed by a nuclear clock, which employs a nuclear transition instead of an atomic shell transition. There is only one known nuclear state that could serve as a nuclear clock using currently available technology, namely, the isomeric first excited state of (229)Th (denoted (229m)Th). Here we report the direct detection of this nuclear state, which is further confirmation of the existence of the isomer and lays the foundation for precise studies of its decay parameters. On the basis of this direct detection, the isomeric energy is constrained to between 6.3 and 18.3 electronvolts, and the half-life is found to be longer than 60 seconds for (229m)Th(2+). More precise determinations appear to be within reach, and would pave the way to the development of a nuclear frequency standard.
The ''island of inversion'' nucleus 32 Mg has been studied by a (t, p) two neutron transfer reaction in inverse kinematics at REX-ISOLDE. The shape coexistent excited 0 þ state in 32 Mg has been identified by the characteristic angular distribution of the protons of the ÁL ¼ 0 transfer. The excitation energy of 1058 keV is much lower than predicted by any theoretical model. The low-ray intensity observed for the decay of this 0 þ state indicates a lifetime of more than 10 ns. Deduced spectroscopic amplitudes are compared with occupation numbers from shell-model calculations. The evolution of shell structure in exotic nuclei as a function of the proton (Z) and neutron (N) number is currently at the center of many theoretical and experimental investigations [1,2]. It has been realized that the interaction of the last valence protons and neutrons, in particular, the monopole component of the residual interaction between those nucleons, can lead to significant shifts in the single-particle energies, leading to the disappearance of classic shell closures and the appearance of new shell gaps [3]. A prominent example is the collapse of the N ¼ 20 shell gap in the neutron-rich oxygen isotopes where instead a new magic shell gap appears for 24 O at N ¼ 16 [4,5]. Recent work showed that the disappearance of the N ¼ 20 shell can be attributed to the monopole effect of the tensor force [3,6,7]. The reduced strength of the attractive interaction between the proton d 5=2 and the neutron d 3=2 orbitals causes the d 3=2 orbital to rise in energy and come closer to the f 7=2 orbital. In regions without pronounced shell closures correlations between the valence nucleons may become as large as the spacing of the single-particle energies. This can thus lead to particle-hole excitations to higher-lying single-particle states enabling deformed configurations to be lowered in energy. This may result in low-lying collective excitations, the coexistence of different shapes at low energies or even the deformation of the ground state for nuclei with the conventional magic number N ¼ 20. Such an effect occurs in the ''island of inversion'', one of most studied regions of exotic nuclei in the nuclear chart. In this region of neutron-rich nuclei around the magic number N ¼ 20 strongly deformed ground states in Ne, Na, and Mg isotopes have been observed [8-11]. Because of the reduction of the N ¼ 20 shell gap, quadrupole correlations can enable low-lying deformed 2p-2h intruder states from the fp shell to compete with spherical normal neutron 0p-0h states of the sd shell. In this situation the promotion of a neutron pair across the N ¼ 20 gap can result in deformed intruder ground states. Consequentially, the competition of two configurations can lead to the coexistence of spherical and deformed 0 þ states in the neutron-rich 30;32 Mg nuclei [12]. Coulomb excitation experiments have shown that 30 Mg has a rather small BðE2Þ value for the 0 þ gs ! 2 þ 1 transition [13,14] placing this nucleus outside the island of inversion. The excited deform...
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