The first-order charge density wave (CDW) phase transition of Er 2 Ir 3 Si 5 is characterized by a crystal structure analysis, and electrical resistivity, magnetic susceptibility and specific heat measurements. The incommensurate CDW is accompanied by a strong lattice distortion, from which it is shown that the CDW resides on zigzag chains of iridium atoms. The CDW transition affects the magnitude of the local magnetic moments on Er 3+ , implying strong coupling between CDW and magnetism. This could account for the observation that magnetic order is suppressed down to at least 0.1 K in the high-quality single crystal presently studied. Any disorder in the crystallinity, as in ceramic material, broadens and suppresses the CDW transition, while magnetic order appears at 2.1 K.
We report on electron spin resonance (ESR) studies of the spin relaxation in Cs2CuCl4. The main source of the ESR linewidth at temperatures T ≤ 150 K is attributed to the uniform DzyaloshinskiiMoriya interaction. The vector components of the Dzyaloshinskii-Moriya interaction are determined from the angular dependence of the ESR spectra using a high-temperature approximation. Both the angular and temperature dependence of the ESR linewidth have been analyzed using a selfconsistent quantum-mechanical approach. In addition analytical expressions based on a quasiclassical picture for spin fluctuations are derived, which show good agreement with the quantumapproach for temperatures T ≥ 2J/kB ≈ 15 K. A small modulation of the ESR linewidth observed in the ac-plane is attributed to the anisotropic Zeeman interaction, which reflects the two magnetically nonequivalent Cu positions.
We present a high-temperature series expansion code for spin-1/2 Heisenberg models on arbitrary lattices. As an example we demonstrate how to use the application for an anisotropic triangular lattice with two independent couplings J 1 and J 2 and calculate the high-temperature series of the magnetic susceptibility and the static structure factor up to 12 th and 10 th order, respectively. We show how to extract effective coupling constants for the triangular Heisenberg model from experimental data on Cs 2 CuBr 4 . Nature of problem: Calculation of thermodynamic properties (magnetic susceptibility and static structure factor) for quantum magnets on arbitrary lattices. A particularly hard problem pose quantum magnets on so frustrated lattice geometries, as they can not be solved efficently by Quantum Monte Carlo methods. Solution method: High-temperature series expansions employing a linked-cluster expansion allow to obtain a high-order series in the inverse temperature for thermodynamic quantities in the thermodynamic limit. The resulting high-temperature series are exact up to the expansion order. We implement the calculation of high-temperature series for the zero-field magnetic susceptibility and static magnetic structure factor for the spin-1/2 Heisenberg model on arbitrary infinite lattices in arbitrary dimension. Program code and examples: http://www.comp-phys.org/lcse/
We present a structural analysis of the substituted system (Ba1−xSrx)CuSi2O6, which reveals a stable tetragonal crystal structure down to 1.5 K. We explore the structural details with lowtemperature neutron and synchrotron powder diffraction, room-temperature and cryogenic highresolution NMR, as well as magnetic-and specific-heat measurements and verify that a structural phase transition into the orthorhombic structure which occurs in the parent compound BaCuSi2O6, is absent for the x = 0.1 sample. Furthermore, synchrotron powder-diffraction patterns show a reduction of the unit cell for x = 0.1 and magnetic measurements prove that the Cu-dimers are preserved, yet with a slightly reduced intradimer coupling Jintra. Pulse-field magnetization measurements reveal the emergence of a field-induced ordered state, tantamount to Bose-Einsteincondensation (BEC) of triplons, within the tetragonal crystal structure of I 41/acd. This material offers the opportunity to study the critical properties of triplon condensation in a simple crystal structure.
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