Sensors play an important part in many aspects of daily life such as infrared sensors in home security systems, particle sensors for environmental monitoring and motion sensors in mobile phones. High-quality optical microcavities are prime candidates for sensing applications because of their ability to enhance light-matter interactions in a very confined volume. Examples of such devices include mechanical transducers, magnetometers, single-particle absorption spectrometers, and microcavity sensors for sizing single particles and detecting nanometre-scale objects such as single nanoparticles and atomic ions. Traditionally, a very small perturbation near an optical microcavity introduces either a change in the linewidth or a frequency shift or splitting of a resonance that is proportional to the strength of the perturbation. Here we demonstrate an alternative sensing scheme, by which the sensitivity of microcavities can be enhanced when operated at non-Hermitian spectral degeneracies known as exceptional points. In our experiments, we use two nanoscale scatterers to tune a whispering-gallery-mode micro-toroid cavity, in which light propagates along a concave surface by continuous total internal reflection, in a precise and controlled manner to exceptional points. A target nanoscale object that subsequently enters the evanescent field of the cavity perturbs the system from its exceptional point, leading to frequency splitting. Owing to the complex-square-root topology near an exceptional point, this frequency splitting scales as the square root of the perturbation strength and is therefore larger (for sufficiently small perturbations) than the splitting observed in traditional non-exceptional-point sensing schemes. Our demonstration of exceptional-point-enhanced sensitivity paves the way for sensors with unprecedented sensitivity.
The ability to detect and size individual nanoparticles with high resolution is crucial to understanding behaviours of single particles and effectively using their strong size-dependent properties to develop innovative products. We report real-time, insitu detection and sizing of single nanoparticles, down to 30 nm in radius, using mode-splitting in a monolithic ultra-high-Q whispering-gallery-mode (WGM) microtoroid resonator. Particle binding splits a WGM into two spectrally shifted resonance modes, forming a self-referenced detection scheme. This technique provides superior noise suppression and enables extracting accurate size information in a single-shot measurement. Our method requires neither labelling of the particles nor apriori information on their presence in the medium, providing an effective platform to study nanoparticles at single particle resolution.
†These authors contributed equally to this work.Controlling and reversing the effects of loss are major challenges in optical systems. For lasers losses need to be overcome by a sufficient amount of gain to reach the lasing threshold. We show how to turn losses into gain by steering the parameters of a system to the vicinity of an exceptional point (EP), which occurs when the eigenvalues and the corresponding eigenstates of a system coalesce. In our system of coupled microresonators, EPs are manifested as the lossinduced suppression and revival of lasing. Below a critical value, adding loss annihilates an existing Raman laser. Beyond this critical threshold, lasing recovers despite the increasing loss, in stark contrast to what would be expected from conventional laser theory. Our results exemplify the counterintuitive features of EPs and present an innovative method for reversing the effect of loss.2 Dissipation is ubiquitous in nature; the states of essentially all physical systems thus have a finite decay time. A proper description of this situation requires a departure from conventional Hermitian models with real eigenvalues and orthogonal eigenstates to non-Hermitian models featuring complex eigenvalues and nonorthogonal eigenstates (1,2,3). When tuning the parameters of such a dissipative system, its complex eigenvalues and the corresponding eigenstates may coalesce, giving rise to a non-Hermitian degeneracy, also called an Exceptional Point (EP) (4). The presence of such an EP has a dramatic effect on the system, leading to nontrivial physics with interesting counterintuitive features such as "resonance trapping" (5), a mode exchange when encircling an EP (6), and a singular topology in the parameter landscape (7). These characteristics can control the flow of light in optical devices with both loss and gain.In particular, waveguides having parity-time symmetry (8), where loss and gain are balanced, have attracted enormous attention (9,10), with effects such as loss-induced transparency (11), unidirectional invisibility (12), and reflectionless scattering (13,14) having been already observed.Theoretical work indicates that EPs give rise to many more intriguing effects when they occur near the lasing regime; for example, enhancement of the laser linewidth (15,16), fast selfpulsations (15), and a pump-induced lasing death (17). Realizing such anomalous phenomena, however, requires moving from waveguides to resonators, which can trap and amplify light resonantly beyond the lasing threshold. With the availability of such devices (18,19), we discuss here the most counterintuitive aspect that close to an EP lasing should be inducible solely by adding loss to a resonator.Our experimental system (20) consists of two directly-coupled silica whispering-gallery-mode resonators (WGMRs) μR 1 and μR 2 , each coupled to a different fiber-taper WG1 and WG2 ( Fig. 1A and sec. S1). The resonance frequencies of the WGMRs were tuned to be the same via thermo-optic effect, and a controllable coupling strength κ was achieve...
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