The microscopic magnetic properties of the Cu02 planes in YBa2Cu306 63 (T, =62 K) have been investigated in Cu and 0 NMR experiments. Unlike the fully oxygenated Y-Ba-Cu-07 (T, =90 K), the various components of the Cu and 0 Knight-shift tensors show strong but identical temperature dependences in the normal state. This supports the picture that there is only one spin component in the Cu02 planes. The spin susceptibility deduced from Knight-shift results shows significant reduction with decreasing temperature in the normal state. The temperature dependences of the nuclear-spin-relaxation rates (1/T& ) are very different for the Cu and the 0 sites. 1/( T& T) at the O sites is nearly proportional to the spin susceptibility. 1/(T& T) at the Cu sites shows a broad peak around 150 K. We discuss these relaxation behaviors based on a model of the dynamical spin susceptibility proposed by Millis, Monien, and Pines.
We report NMR measurements of the nuclear relaxation rate at all copper and oxygen sites in magnetically aligned powder samples of YB^CM^OI.Comparison of the oxygen and copper relaxation reveals a characteristic temperature greater than T c . The copper relaxation rate is enhanced by antiferromagnetic copper spin fluctuations which are undiminished in the superconducting state. The absence of a coherence peak indicates that the superconductive pairing is not of the conventional BCS type. PACS numbers: 74.70.Vy, 74.30.Gn, 76.60.Es, 76.60.Jx The nature of spin fluctuations in the hightemperature superconducting copper oxides and their possible role in superconductive pairing are problems of central importance in our understanding of these materials. Nuclear-magnetic-relaxation-rate (TT l ) measurements microscopically probe spin dynamics at the atomic sites and so provide crucial insight into this question. Accordingly we have measured the relaxation rate at all oxygen and copper sites in magnetically aligned powders l of YBa2Cu307. Comparison of the copper and oxygen NMR relaxation rates shows that the large magnitude of the copper relaxation rate in the normal state is due to antiferromagnetic copper spin fluctuations and that these antiferromagnetic spin fluctuations persist into the superconducting state. The behavior of these fluctuations changes 0.1 D 0.01 0.001 -I
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