Facing the ever-growing demand for data storage will most probably require a new paradigm. Magnetic skyrmions are anticipated to solve this issue as they are arguably the smallest spin textures in magnetic thin films in nature. We designed cobalt-based multilayered thin films where the cobalt layer is sandwiched between two heavy metals providing additive interfacial Dzyaloshinskii-Moriya interactions, which reach about 2 mJ/m 2 in the case of the Ir|Co|Pt multilayers. Using a magnetization-sensitive scanning x-ray transmission microscopy technique, we imaged magnetic bubble-like domains in these multilayers. The study of their behavior in magnetic field allows us to conclude that they are actually magnetic skyrmions stabilized by the Dzyaloshinskii-Moriya interaction. This discovery of stable skyrmions at room temperature in a technologically relevant material opens the way for device applications in a near future.A major societal challenge is related to the continually increasing quantity of information to process and store. The hard disk drives, in which information is encoded magnetically, allow nowadays the storage of zettabytes (10 21 ) of information, but this technology should soon reach its limits. An up-and-coming avenue has been opened by the discovery of magnetic skyrmions [1], i.e. spin windings that can be localized within a diameter of a few nanometers and can move like particles [2]. These magnetic solitons, remarkably robust against defects due to the topology of their magnetic texture [3], are promising for being the ultimate magnetic bits to carry and store information. The topology of the skyrmions also appears to further underlie other important features such as their current-induced motion induced by small dc currents that is crucial for real applications but also the existence of a specific component in Hall Effect [4][5][6] that can be used advantageously for an electrical read-out of the information carried by nano-scale skyrmions. We proposed recently that these skyrmions could be used in future storage devices and information processing [2].The existence of skyrmion spin configuration has been predicted theoretically about thirty years ago [1] but it was only recently that skyrmion lattices have been observed in crystals with noncentrosymmetric lattices, e.g. B20 crystallographic structure in MnSi [7][8][9] FeCoSi [10] or FeGe [5] crystals. In 2011, skyrmions have also been identified in single ultrathin ferromagnetic films with out-of-plane magnetization (Fe and FePd) deposited on a heavy metal substrate such as Ir(1 1 1) [11,12]. Thin magnetic films appear to be more compatible with technological developments, though the observation of skyrmions in thin films has been limited up to now to low temperature and also needs, in some cases, the presence of a large applied magnetic field [12]. The study of these new magnetic phases associated with chiral interactions has generated a
We present an innovative approach to the production of single-crystal iron oxide nanorings employing a solution-based route. Single-crystal hematite (alpha-Fe2O3) nanorings were synthesized using a double anion-assisted hydrothermal method (involving phosphate and sulfate ions), which can be divided into two stages: (1) formation of capsule-shaped alpha-Fe2O3 nanoparticles and (2) preferential dissolution along the long dimension of the elongated nanoparticles (the c axis of alpha-Fe2O3) to form nanorings. The shape of the nanorings is mainly regulated by the adsorption of phosphate ions on faces parallel to c axis of alpha-Fe2O3 during the nanocrystal growth, and the hollow structure is given by the preferential dissolution of the alpha-Fe2O3 along the c axis due to the strong coordination of the sulfate ions. By varying the ratios of phosphate and sulfate ions to ferric ions, we were able to control the size, morphology, and surface architecture to produce a variety of three-dimensional hollow nanostructures. These can then be converted to magnetite (Fe3O4) and maghemite (gamma-Fe2O3) by a reduction or reduction-oxidation process while preserving the same morphology. The structures and magnetic properties of these single-crystal alpha-Fe2O3, Fe3O4, and gamma-Fe2O3 nanorings were characterized by various analytical techniques. Employing off-axis electron holography, we observed the classical single-vortex magnetic state in the thin magnetite nanorings, while the thicker rings displayed an intriguing three-dimensional magnetic configuration. This work provides an easily scaled-up method for preparing tailor-made iron oxide nanorings that could meet the demands of a variety of applications ranging from medicine to magnetoelectronics.
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