Magnetic skyrmions are arguably the smallest stable magnetic configuration in films, and therefore could be the ultimate magnetic storage bit [1,2] . They have also triggered a wide interest due to the new fundamental phenomena related to their topology . Numerical simulations have shown that the interfacial Dzyaloshinskii-Moriya interaction (DMI) can stabilize such skyrmions in nanoscale disks or tracks for a rather large range of DMI amplitudes for which the skyrmion can either be the ground state or metastable relative to the uniform state [4,5,6] . Here, we demonstrate experimentally the presence of skyrmions in metallic multilayers structures engineered to exhibit a strong DMI interaction . In this work, beyond the study of skyrmions in thin films [3], we focus our investigation on sputtered multilayers with vertical magnetization consisting of stacks of trilayers composed of 0 .6-nm-thick Co layers sandwiched between 5d transition metal layers, namely Pt, Ir and W . Asymmetric sandwiches were designed in order to introduce additive DMI from the top and bottom interfaces of Co [2,5,6] while also obtaining a considerable perpendicular magnetic anisotropy . We will present our results on two types of metallic multilayers grown at room temperature: |Pt10|-Co0 .6|Pt1|{Co0 .6|Pt1}x10|Pt3 and |Pt10|Co0 .6|Pt1|{Ir1|Co0 .6|Pt1}x10|Pt3 (thickness in nm) . The magnetic anisotropy is determined using standard magnetometry, while the DMI amplitude is estimated by two original methods . Based on detailed mapping of the magnetization obtained using scanning transmission X-ray microscopy (STXM) combined with the XMCD effect, STXM allows the magnetic imaging of patterned structures in a non-invasive way with nanoscale resolution (<50 nm) [7] . We acquired such images at different perpendicular magnetic fields in both symmetric Pt|Co|Pt and asymmetric Pt|Co|Ir multilayers [8] . From the analysis of the magnetic domain configurations, either at zero field after demagnetization (not shown) or following the evolution of the size of bubbles with perpendicular magnetic field (Figure 1), we evaluate consistently a DMI amplitude D as large as 2 mJ/ m 2 in Pt|Co|Ir . The process for estimating the skyrmion radius is displayed in Figure 2 . A direct consequence of having such a large DMI is that the bubble-like domains that we have identified are indeed isolated magnetic skyrmions . In micromagnetic simulations, trivial bubbles (winding number equal to zero) are not stable and vanish in a few nanoseconds or less, while skyrmions (winding number equal to one) are stable . The good agreement of the size dependence as well as the stability of the bubble domains is strong evidence that these domains are, in fact, skyrmions . The value of D is further confirmed by studying the typical width of the worm domains, which are observed at zero magnetic field, indicating consistency in the analysis .In conclusion, we demonstrate the presence, at room temperature, of skyrmions stabilized by interfacial DMI in metallic multilayers, opening the...
Since the discovery of ferromagnetic two-dimensional (2D) van der Waals (vdW) crystals, significant interest on such 2D magnets has emerged, inspired by their appealing physical properties and integration with other 2D family for unique heterostructures. In known 2D magnets, spin-orbit coupling (SOC) stabilizes perpendicular magnetic anisotropy down to one or a few monolayers. Such a strong SOC could also lift the chiral degeneracy, leading to the formation of topological magnetic textures such as skyrmions through the Dzyaloshinskii-Moriya interaction (DMI). Here, we report the experimental observation of Néel-type chiral magnetic skyrmions and their lattice (SkX) formation in a vdW ferromagnet Fe 3 GeTe 2 (FGT). We demonstrate the ability to drive an individual skyrmion by short current pulses along a vdW heterostructure, FGT/h-BN, as highly required for any skyrmion-based spintronic device. Using first principle calculations supported by experiments, we unveil the origin of DMI being the interfaces with oxides, which then allows us to engineer vdW heterostructures for desired chiral states. Our finding opens the door to topological spin textures in the 2D vdW magnet and their potential device application.
Whiteness arises from the random scattering of incident light from disordered structures. [1] Opaque white materials have to contain a sufficiently large number of scatterers and therefore usually require thicker, material-rich nanostructures than structural color arising from the coherent interference of light. [2,3] In nature, bright white appearance arises from the dense arrays of pterin pigments in pierid butterflies, [4] guanine crystals in spiders, [5] or leucophore cells in the flexible skin of cuttlefish. [6] A striking example of such whiteness is found in the chitinous networks of white beetles, e.g., Lepidiota stigma and Cyphochilus sp. [7][8][9] Previous research investigating these beetle structures has shown that the chitinous network is one of the most strongly scattering materials in nature, and therefore the question arises whether this structure is evolutionary optimized for strong scattering while minimizing the Most studies of structural color in nature concern periodic arrays, which through the interference of light create color. The "color" white however relies on the multiple scattering of light within a randomly structured medium, which randomizes the direction and phase of incident light. Opaque white materials therefore must be much thicker than periodic structures. It is known that flying insects create "white" in extremely thin layers. This raises the question, whether evolution has optimized the wing scale morphology for white reflection at a minimum material use. This hypothesis is difficult to prove, since this requires the detailed knowledge of the scattering morphology combined with a suitable theoretical model. Here, a cryoptychographic X-ray tomography method is employed to obtain a full 3D structural dataset of the network morphology within a white beetle wing scale. By digitally manipulating this 3D representation, this study demonstrates that this morphology indeed provides the highest white retroreflection at the minimum use of material, and hence weight for the organism. Changing any of the network parameters (within the parameter space accessible by biological materials) either increases the weight, increases the thickness, or reduces reflectivity, providing clear evidence for the evolutionary optimization of this morphology. amount of employed material, thus reducing the weight of the organism. The brilliant white reflection from Cyphochilus beetles is assumed to be important for camouflage among white fungi and in a shady environment.In contrast to periodic photonic materials, for which the optical response is straightforward to calculate, the reflection of light from such disordered network morphologies requires a detailed knowledge of local geometry. [2,3,9,10] For these complex cases, the validity of the diffusion approximation is limited, since single scattering elements are difficult to be identified. [7] To fully understand the correlation between the structure and (optical) properties of complex materials, the detailed real-space structure in combination with a s...
anisotropy (PMA). In ultrathin films, skyrmions can exhibit sub-nanometer scale size [8][9][10][11] and move in response to an applied current with velocities exceeding 100 m s -1 [5] in a controllable [12,13] and reliable [13] way. Therefore, they promise great technological utility for racetracktype memories, [14] logic gates, [15] probabilistic computing, [16] and neuromorphic devices, [17] for which they have to be readily created and manipulated. Homochiral skyrmions can be stabilized by the Dzyaloshinkii-Moriya interaction (DMI) [18,19] in materials with strong spin-orbit coupling and broken inversion symmetry. Since asymmetric multilayer stacks of a ferromagnet and a heavy metal [5][6][7] possess DMI and can also exhibit large current-induced spin-orbit torques that can provide an efficient means to create and manipulate skyrmions, [20][21][22] these systems are now a central focus of current research. Magnetic skyrmions can exist as isolated topological excitations, [23,24] or as ordered arrays (hexagonal lattice) comprising the magnetic ground state, [2,5] depending on material and Magnetic skyrmions promise breakthroughs in future memory and computing devices due to their inherent stability and small size. Their creation and current driven motion have been recently observed at room temperature, but the key mechanisms of their formation are not yet well-understood. Here it is shown that in heavy metal/ferromagnet heterostructures, pulsed currents can drive morphological transitions between labyrinth-like, stripe-like, and skyrmionic states. Using high-resolution X-ray microscopy, the spin texture evolution with temperature and magnetic field is imaged and it is demonstrated that with transient Joule heating, topological charges can be injected into the system, driving it across the stripe-skyrmion boundary. The observations are explained through atomistic spin dynamic and micromagnetic simulations that reveal a crossover to a global skyrmionic ground state above a threshold magnetic field, which is found to decrease with increasing temperature. It is demonstrated how by tuning the phase stability, one can reliably generate skyrmions by short current pulses and stabilize them at zero field, providing new means to create and manipulate spin textures in engineered chiral ferromagnets. Magnetic SkyrmionsThe ORCID identification number(s) for the author(s) of this article can be found under https://doi.
Spin waves offer intriguing novel perspectives for computing and signal processing, since their damping can be lower than the Ohmic losses in conventional CMOS circuits. For controlling the spatial extent and propagation of spin waves on the actual chip, magnetic domain walls show considerable potential as magnonic waveguides. However, low-loss guidance of spin waves with nanoscale wavelengths, in particular around angled tracks, remains to be shown. Here we experimentally demonstrate that such advanced control of propagating spin waves can be obtained using natural features of magnetic order in an interlayer exchange-coupled, anisotropic ferromagnetic bilayer. Using Scanning Transmission X-Ray Microscopy, we image generation of spin waves and their propagation across distances exceeding multiple times the wavelength, in extended planar geometries as well as along one-dimensional domain walls, which can be straight and curved. The observed range of wavelengths is between 1 µm and 150 nm, at corresponding excitation frequencies from 250 MHz to 3 GHz. Our results show routes towards practical implementation of magnonic waveguides employing domain walls in future spin wave logic and computational circuits.
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