Superconductivity often occurs close to broken-symmetry parent states and is especially common in doped magnetic insulators 1 . When twisted close to a magic relative orientation angle near !°, bilayer graphene has flat moiré superlattice minibands that have emerged as a rich and highly tunable source of strong correlation physics 2-5 , notably the appearance of superconductivity close to interaction-induced insulating states. Here we report on the fabrication of bilayer graphene devices with exceptionally uniform twist angles. We show that the reduction in twist angle disorder reveals insulating states at all integer occupancies of the four-fold spin/valley degenerate flat conduction and valence bands, i.e. at moiré band filling factors # = %, ±!, ±(, ±), and superconductivity below critical temperatures as high as ~ 3 K close to -2 filling. We also observe three new superconducting domes at much lower temperatures close to the # = % and # = ±! insulating states. Interestingly, at # = ±! we find states with non-zero Chern numbers. For # = −! the insulating state exhibits a sharp hysteretic resistance enhancement when a perpendicular magnetic field above 3.6 tesla is applied, consistent with a field driven phase transition. Our study shows that symmetry-broken states, interaction driven insulators, and superconducting domes are common across the entire moiré flat bands, including near charge neutrality.
Flat-bands in magic angle twisted bilayer graphene (MATBG) have recently emerged as a rich platform to explore strong correlations, superconductivity and magnetism. However, the phases of MATBG in magnetic field, and what they reveal about the zero-field phase diagram remain relatively unchartered. Here we use magnetotransport and Hall measurements to reveal a rich sequence of wedge-like regions of quantized Hall conductance with Chern numbers C = ±1, ±2, ±3, ±4 which nucleate from integer fillings of the moiré unit cell 𝜈 = ±3, ±2, ±1, 0 correspondingly. We interpret these phases as spin and valley polarized Chern insulators, equivalent to quantum Hall ferromagnets. The exact sequence and correspondence of Chern numbers and filling factors suggest that these states are driven directly by electronic interactions which specifically break time-reversal symmetry in the system. We further study quantum magneto-oscillation in the yet unexplored higher energy dispersive bands with a Rashba-like dispersion. Analysis of Landau level crossings enables a parameter-free comparison to a newly derived "magic series" of level crossings in magnetic field and provides constraints on the parameters w0 and w1 of the Bistritzer-MacDonald MATBG Hamiltonian. Overall, our data provides direct insights into the complex nature of symmetry breaking in MATBG and allows for quantitative tests of the proposed microscopic scenarios for its electronic phases.
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.