Recent progress in laser-based high-repetition rate extreme ultraviolet (EUV) lightsources and multidimensional photoelectron spectroscopy enable the build-up of a new generation of time-resolved photoemission experiments. Here, we present a setup for time-resolved momentum microscopy driven by a 1 MHz femtosecond EUV table-top light source optimized for the generation of 26.5 eV photons. The setup provides simultaneous access to the temporal evolution of the photoelectron´s kinetic energy and in-plane momentum. We discuss opportunities and limitations of our new experiment based on a series of static and time-resolved measurements on graphene.
Coherent extreme ultraviolet (XUV) radiation produced by table-top high-harmonic generation (HHG) sources provides a wealth of possibilities in research areas ranging from attosecond physics to high resolution coherent diffractive imaging. However, it remains challenging to fully exploit the coherence of such sources for interferometry and Fourier transform spectroscopy (FTS). This is due to the need for a measurement system that is stable at the level of a wavelength fraction, yet allowing a controlled scanning of time delays. Here we demonstrate XUV interferometry and FTS in the 17-55 nm wavelength range using an ultrastable common-path interferometer suitable for high-intensity laser pulses that drive the HHG process. This approach enables the generation of fully coherent XUV pulse pairs with sub-attosecond timing variation, tunable time delay and a clean Gaussian spatial mode profile. We demonstrate the capabilities of our XUV interferometer by performing spatially resolved FTS on a thin film composed of titanium and silicon nitride.A well-known feature of high-harmonic generation (HHG) is broadband spectra in the XUV and soft X-ray regions [1][2][3]. This radiation is typically emitted in a train of attosecond pulses with excellent spatial and temporal coherence, as shown in various interferometric and spectroscopic measurements [4][5][6][7][8][9][10][11][12]. As a result, interferometry with high harmonics found important applications in e.g. Molecular Orbital Tomography [13], in wavefront reconstruction [14] and electric field characterization [15] of high harmonics. Recently, interferometry with high harmonics provided added value to coherent diffractive imaging (CDI) [16,17] using the full high harmonics bandwidth and photon flux. However, in the extreme ultraviolet (XUV) spectral range, interferometry and Fourier transform spectroscopy (FTS) are challenging due to the high stability requirements of the interferometer itself. Two main types of HHG interferometers have been devised. In one scheme, the near-infrared fundamental driving pulse is split into two phase-locked pulses with an adjustable time delay, and this pulse pair is subsequently used for HHG [5,[7][8][9]. Although this method has been successfully used it is typically limited by the stability of the optical interferometer. The other scheme is based on wavefront division, whereby one HHG beam is divided into two phase-locked sources by a piezo-mounted split mirror. This configuration allows more stable interferometry [10,[18][19][20][21], but results in two beams with different spatial profiles and strong diffraction effects due to the hard edge of the split mirror. Wavefront division interferometry is also less flexible when one would like to change the intensity ratio between the two beams.In this letter we present XUV interferometry using a novel ultrastable common-path interferome-1 arXiv:1607.02386v2 [physics.optics]
We present energy-resolved photoelectron momentum maps for orbital tomography that have been collected with a novel and efficient time-of-flight momentum microscopy setup. This setup is combined with a 0.5 MHz table-top femtosecond extremeultraviolet light source, which enables unprecedented speed in data collection and paves the way towards time-resolved orbital imaging experiments in the future. Moreover, we take a significant step forward in the data analysis procedure for orbital imaging, and present a sparsity-driven approach to the required phase retrieval problem, which uses only the number of non-zero pixels in the orbital. Here, no knowledge of the object support is required, and the sparsity number can easily be determined from the measured data. Used in the relaxed averaged alternating reflections algorithm, this sparsity constraint enables fast and reliable phase retrieval for our experimental as well as noise-free and noisy simulated photoelectron momentum map data.
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