We would like to acknowledge the support and successful cooperation of NASA and CNES in the development and operation of CALIPSO and the advocacy of Gérard Mégie for the mission. We thank Bill Hunt and the team at Ball Aerospace for CALIOP and payload integration; the teams at SODERN and Thales Alenia Space for the IIR and platform integration, respectively; the operations teams at NASA and CNES; and the support of the ASDC and ICARE data centers, who all made essential contributions to the success of the CALIPSO mission. The work described in "The occurrence of marine stratus and stratocumulus" was carried out by T. Kubar in collaboration with D. E.
Odin is a 250 kg class satellite built in co-operation between Sweden, Canada, France, and Finland and launched in February 2001. It carries two instruments: a 4-band sub-millimetre radiometer used for both astronomy and atmospheric science and an optical spectrometer and infrared imaging system for purely atmospheric observations. As part of the joint mission Odin will observe the atmospheric limb for 50% of the observation time producing profiles of many species of interest in the middle atmosphere with a vertical resolution of 12 km. These species include, among others, ozone, nitrogen dioxide, chlorine monoxide, nitric acid, water vapour, and nitrous oxide. An overview of the mission and the planned measurements is given. PACS Nos.: 42.68Mj, 94.10Dy, 95.55Fw
The optical spectrograph and infrared imager system (OSIRIS) on board the Odin spacecraft is designed to retrieve altitude profiles of terrestrial atmospheric minor species by observing limb-radiance profiles. The grating optical spectrograph (OS) obtains spectra of scattered sunlight over the range 280-800 nm with a spectral resolution of approximately 1 nm. The Odin spacecraft performs a repetitive vertical limb scan to sweep the OS 1 km vertical field of view over selected altitude ranges from approximately 10 to 100 km. The terrestrial absorption features that are superimposed on the scattered solar spectrum are monitored to derive the minor species altitude profiles. The spectrograph also detects the airglow, which can be used to study the mesosphere and lower thermosphere. The other part of OSIRIS is a three-channel infrared imager (IRI) that uses linear array detectors to image the vertical limb radiance over an altitude range of approximately 100 km. The IRI observes both scattered sunlight and the airglow emissions from the oxygen infrared atmospheric band at 1.27 µm and the OH (3-1) Meinel band at 1.53 µm. A tomographic inversion technique is used with a series of these vertical images to derive the two-dimensional distribution of the emissions within the orbit plane.Résumé : Le système de spectrographie optique et d'imagerie infrarouge (OSIRIS) à bord du satellite Odin est conçu pour enregistrer les profils en altitude des éléments mineurs de l'atmosphère en observant les profils de radiance du limbe. Le spectrographe optique à réseau (OS) obtient les spectres de la lumière solaire diffusée sur le domaine entre 280-800 nm, avec une résolution spatiale approximative de 1 nm. Le satellite Odin balaye verticalement le limbe de façon répétée, de telle sorte que l'ouverture verticale de 1 km du OS parcoure les domaines voulus entre 10 et 100 km. Nous analysons les spectres solaires diffusés en superposition avec les caractéristiques terrestres d'absorption, afin de déterminer les profils en altitude des éléments mineurs de l'atmosphère. Le spectrographe détecte aussi la luminescence nocturne atmosphérique qui peut être utilisé pour étudier la mésosphère et la thermosphère. L'autre partie d'OSIRIS est un imageur infrarouge (IRI) à trois canaux qui utilise une banque linéaire de détecteurs pour imager la radiance du limbe sur un domaine d'altitude d'approximativement 100 km. L'IRI observe à la fois la lumière solaire diffusée et les émissions de luminescence nocturne atmospérique provenant de la bande infrarouge de l'oxygène atmosphérique à 1.27 µm et la bande de Meinel de l'OH (3-1) à 1.53 µm. Nous utilisons une technique d'inversion tomographique avec une série de ces images verticales pour obtenir la distribution bidimensionnelle des émissions à l'intérieur de l'orbite.[Traduit par la Rédaction] Can.
The global tropospheric distributions of seven important sulfur species were simulated with a global three‐dimensional chemistry‐transport model (IMAGES). Surface emission and deposition velocity maps were established for use as lower boundary conditions in the model. While anthropogenic SO2 emissions are by far the largest sulfur source in the northern midlatitudes, reduced sulfur compounds, notably dimethyl sulfide (DMS) predominate over most remote areas. Simulations were performed for the present‐day (∼ 1985) atmosphere. The calculated distributions are compared with available observations. The model results are found to be generally within a factor of (at most) 2–3 of long‐term observations. Comparison with campaign measurements is more difficult, mostly due to the strong dependence of sulfur species concentrations on local meteorological conditions. The results, however, indicate the need for future model refinements, especially with respect to biogenic emission estimates and parameterization of cloud processes. A sensitivity study is presented to discuss the uncertainties of the results related to several parameters (the decoupling of wet scavenging and convective transport for soluble species, volcanoes emission and deposition velocities). Results are also discussed in terms of global budgets and related variables and processes. Around 125 Tg S/yr of non‐sea‐salt (nss) sulfur compounds (DMS, CS2, H2S, COS, and SO2) are injected into the atmosphere. The balance is mainly maintained by nss‐sulfates wet and dry deposition, and by SO2 dry deposition (94% of total sulfur deposition). It is found that DMS oxidation represents the main contribution to SO2 chemical production (80% of the chemical sources), and that the major sink of SO2 is provided by in‐cloud oxidation (90% of the chemical sinks), under the assumption that all SO2 incorporated into clouds is oxidized. The calculated annual wet deposition of sulfates reaches 3 g S m−2 yr−1 over Europe and North America, while it is usually lower than 0.5 g S m−2 yr−1 in remote parts of the world. Estimations for the global lifetimes are 0.9 day for DMS, 4 days for CS2, 2.2 days for H2S, 0.6 day for SO2, 0.18 day for DMSO, 6.1 days for MSA, and 4.7 days for nss‐sulfates.
Between November 1999 and April 2000, two major field experiments, the Stratospheric Aerosol and Gas Experiment (SAGE) III Ozone Loss and Validation Experiment (SOLVE) and the Third European Stratospheric Experiment on Ozone (THESEO 2000), collaborated to form the largest field campaign yet mounted to study Arctic ozone loss. This international campaign involved more than 500 scientists from over 20 countries. These scientists made measurements across the high and middle latitudes of the Northern Hemisphere. The main scientific aims of SOLVE/THESEO 2000 were to study (1) the processes leading to ozone loss in the Arctic vortex and (2) the effect on ozone amounts over northern midlatitudes. The campaign included satellites, research balloons, six aircraft, ground stations, and scores of ozonesondes. Campaign activities were principally conducted in three intensive measurement phases centered on early December 1999, late January 2000, and early March 2000. Observations made during the campaign showed that temperatures were below normal in the polar lower stratosphere over the course of the 1999–2000 winter. Because of these low temperatures, extensive polar stratospheric clouds (PSC) formed across the Arctic. Large particles containing nitric acid trihydrate were observed for the first time, showing that denitrification can occur without the formation of ice particles. Heterogeneous chemical reactions on the surfaces of the PSC particles produced high levels of reactive chlorine within the polar vortex by early January. This reactive chlorine catalytically destroyed about 60% of the ozone in a layer near 20 km between late January and mid‐March 2000, with good agreement being found between a number of empirical and modeling studies. The measurements made during SOLVE/THESEO 2000 have improved our understanding of key photochemical parameters and the evolution of ozone‐destroying forms of chlorine.
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