The one-dimensional electronic derealization that results from the solid-state polymerization of diacetylenes produces a dramatic enhancement of the optical nonlinearities of these compounds. The third-order susceptibilities of the polymerized crystals reach very high values comparable to those of inorganic semiconductors.
Photodissociation of hydrogen iodide on the surface of large argon clusters: The orientation of the librational wave function and the scattering from the cluster cage
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