Fine structure in the region of the isoscalar giant quadrupole resonance (ISGQR) in 58Ni, 89Y, 90Zr, 120Sn, 166Er, and 208Pb has been observed in high-energy-resolution ( E1/2 35–50 keV) inelastic proton scattering measurements at E0 = 200 MeV at iThemba LABS. Calculations of the corresponding quadrupole excitation strength functions performed within models based on the random-phase approximation (RPA) reveal similar fine structure when the mixing of one-particle one-hole states with two-particle two-hole states is taken into account. A detailed comparison of the experimental data is made with results from the quasiparticle-phonon model (QPM) and the extended time-dependent Hartree-Fock (ETDHF) method. For 208Pb, additional theoretical results from second RPA and the extended theory of finite Fermi systems (ETFFS) are discussed. A continuous wavelet analysis of the experimental and the calculated spectra is used to extract dominant scales characterizing the fine structure. Although the calculations agree with qualitative features of these scales, considerable differences are found between the model and experimental results and amongst different models. Within the framework of the QPM and ETDHF calculations it is possible to decompose the model spaces into subspaces approximately corresponding to different damping mechanisms. It is demonstrated that characteristic scales mainly arise from the collective coupling of the ISGQR to low-energy surface vibrations
The epidermal permeability barrier forms late in gestation, coincident with decreased lipid synthesis, increased lipid processing, and development of a mature, multi-layered stratum corneum. Prior studies have shown that changes in the epidermal Ca++ gradient in vivo regulate lamellar body secretion and lipid synthesis, and modulations in extracellular Ca++ in vitro also regulate keratinocyte differentiation. We asked here whether a Ca++ gradient forms in fetal epidermis in utero, and whether its emergence correlates with key developmental milestones of barrier formation and stratum corneum development. Using either ion precipitation or proton induced X-ray emission analysis of fetal mouse and rat skin, we showed that a Ca++ gradient is not present at gestational days 16-18, prior to barrier formation, and that a gradient forms coincident with the emergence of barrier competence (day 19, mouse; day 20, rat) prior to birth. These results are consistent with a role for Ca++ in the regulation of key metabolic events leading to barrier formation. Whether the calcium gradient is formed actively or passively remains to be determined.
The ability to inject dopant atoms with high spatial resolution, flexibility in dopant species, and high single ion detection fidelity opens opportunities for the study of dopant fluctuation effects and the development of devices in which function is based on the manipulation of quantum states in single atoms, such as proposed quantum computers. The authors describe a single atom injector, in which the imaging and alignment capabilities of a scanning force microscope ͑SFM͒ are integrated with ion beams from a series of ion sources and with sensitive detection of current transients induced by incident ions. Ion beams are collimated by a small hole in the SFM tip and current changes induced by single ion impacts in transistor channels enable reliable detection of single ion hits. They discuss resolution limiting factors in ion placement and processing and paths to single atom ͑and color center͒ array formation for systematic testing of quantum computer architectures in silicon and diamond.
Fine structure in the energy region of the isoscalar giant quadrupole resonance in nuclei is observed in high-resolution proton scattering experiments at iThemba LABS over a wide mass range. A novel method based on wavelet transforms is introduced for the extraction of scales characterizing the fine structure. A comparison with microscopic model calculations including two-particle two-hole (2p2h) degrees of freedom identifies the coupling to surface vibrations as the main source of the observed scales. A generic pattern is also found for the stochastic coupling to the background of the more complex states.
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