At relatively low temperature (e.g, -30 oC), most flexible supercapacitors that work well at room temperature will lose their stretchability due to the poor cold intolerance of conventional electrolytes and...

We summarized the progress in the synthesis, doping and modification strategies of GQDs and the development and application of GQDs in energy storage and conversion devices.

The construction of multidimensional, diversified microsupercapacitors (MSC) is urgently needed for fast-changing flexible and wearable microelectronics, which still meets the challenges of tedious construction and difficult integration. Herein, a laser direct writing strategy has been developed for the one-step preparation of multiscale MSCs from editable macro-supercapacitors. The microstructured supercapacitors with predefined multiscale shapes not only maintain the high capacitance performance and stability but also display the tensile properties in arbitrary direction. The heat-treated ion liquid-modified reduced graphene oxide guarantees the thermal stability of an electrode material during laser cutting, and its high ion-accessible surface area improves the capacitance performance of the supercapacitor. The as-fabricated MSC demonstrates a wide voltage window (0–3 V), high areal specific capacitance (27.4 mF cm–2), and high energy density (32.1 μW h cm–2), which are far higher than those of most reported articles. Notably, the editable supercapacitors can imitate the stereo paper cutting to achieve an arbitrary one-dimensional to three-dimensional configuration, promising for various portable, stretchable, and wearable devices.