When a heavy atomic nucleus splits (fission), the resulting fragments are observed to emerge spinning 1 ; this phenomenon has been a mystery in nuclear physics for over 40 years 2,3 . The internal generation of six or seven units of angular momentum in each fragment is particularly puzzling for systems that start with zero, or almost zero, spin. There are currently no experimental observations that enable decisive discrimination between the many competing theories for the mechanism that generates the angular momentum [4][5][6][7][8][9][10][11][12] . Nevertheless, the consensus is that excitation of collective vibrational modes generates the intrinsic spin before the nucleus splits (pre-scission). Here we show that there is no significant correlation between the spins of the fragment partners, which leads us to conclude that angular momentum in fission is actually generated after the nucleus splits (post-scission). We present comprehensive data showing that the average spin is strongly mass-dependent, varying in saw-tooth distributions. We observe no notable dependence of fragment spin on the mass or charge of the partner nucleus, confirming the uncorrelated post-scission nature of the spin mechanism. To explain these observations, we propose that the collective motion of nucleons in the ruptured neck of the fissioning system generates two independent torques, analogous to the snapping of an elastic band. A parameterization based on occupation of angular momentum states according to statistical theory describes the full range of experimental data well. This insight into the role of spin in nuclear fission is not only important for the fundamental understanding and theoretical description of fission, but also has consequences for the γ-ray heating problem in nuclear reactors 13,14 , for the study of the structure of neutron-rich isotopes 15,16 , and for the synthesis and stability of super-heavy elements 17,18 .

Prompt-fission γ -ray spectra (PFGS) have been measured for the 238 U(n, f ) reaction using fast neutrons produced by the LICORNE directional neutron source. Fission events were detected with an ionization chamber containing actinide samples placed in the neutron beam, and the coincident prompt-fission γ rays were measured using a number of LaBr 3 scintillation detectors and a cluster of nine phoswich detectors from the PARIS array. Prompt-fission γ rays (PFGs) were discriminated from prompt-fission neutrons using the time-of-flight technique over distances of around 35 cm. PFG emission spectra were measured at two incident neutron energies of 1.9 and 4.8 MeV for 238 U(n, f )andalsofor 252 Cf (sf ) as a reference. Spectral characteristics of PFG emission, such as mean γ multiplicity and average total γ -ray energy per fission, as well as the average γ -ray energy, were extracted. The sensitivity of these results to the width of the time window and the type of spectral unfolding procedure used to correct for the detector responses was studied. Iteration methods were found to be more stable in low-statistics data sets. The measured values at E n = 1.9 MeV were found to be the mean γ multiplicity M γ = 6.54 ± 0.19, total released energy per fission E γ,tot = 5.25 ± 0.20 MeV, and the average γ -ray energy ǫ γ = 0.80 ± 0.04 MeV. Under similar conditions, the values at E n = 4.8 MeV were measured to be M γ = 7.31 ± 0.46, E γ,tot = 6.18 ± 0.65 MeV, and ǫ γ = 0.84 ± 0.11 MeV.

K. HADYŃSKA-KLȨK et al. PHYSICAL REVIEW C 97, 024326 (2018) A Coulomb-excitation experiment to study electromagnetic properties of 42 Ca was performed using a 170-MeV calcium beam from the TANDEM XPU facility at INFN Laboratori Nazionali di Legnaro. γ rays from excited states in 42 Ca were measured with the AGATA spectrometer. The magnitudes and relative signs of ten E2matrix elements coupling six low-lying states in 42 Ca, including the diagonal E2 matrix elements of 2 + 1 and 2 + 2 states, were determined using the least-squares code GOSIA. The obtained set of reduced E2 matrix elements was analyzed using the quadrupole sum rule method and yielded overall quadrupole deformation for 0 + 1,2 and 2 + 1,2 states, as well as triaxiality for 0 + 1,2 states, establishing the coexistence of a weakly deformed ground-state band and highly deformed slightly triaxial sideband in 42 Ca. The experimental results were compared with the state-of-the-art large-scale shell-model and beyond-mean-field calculations, which reproduce well the general picture of shape coexistence in 42 Ca.

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