PACS. 42.50.Gy -Effects of atomic coherence on propagation, absorption, and amplification of light; electromagnetically induced transparency and absorption. PACS. 32.70.Jz -Line shapes, widths, and shifts. PACS. 42.50.Md -Optical transient phenomena: quantum beats, photon echo, free-induction decay, dephasings and revivals, optical nutation, and self-induced transparency.Abstract.-In a thin cell of dilute vapour, the absorption spectrum exhibits sub-Doppler features due to the relative enhancement of the slow atom contribution, with respect to the transient nature of the interaction with moving atoms. For a two-level system in the linear regime, the narrowest response is predicted to be found for a λ/2 thickness, as an effect of the coherent character of the dipole response as early described by Romer and Dicke (Phys. Rev., 99 (1955) 532) in the microwave regime. We report here on the direct observation of this effect in the optical regime in an ultra-thin vapour cell. This effect is shown to vanish for a thickness equal to λ, and a revival is observed at 3λ/2, as expected from the predicted λ-periodicity. The experiment is performed on the D1 resonance line of Cs vapour (λ = 894 nm), in a specially designed cell, whose thickness varies locally.
Since the recent realization of extremely thin vapour cells (local thickness: 20-1000 nm), we investigate the optical properties of these 1-D confined vapours. Aside from their interest for Doppler-free spectroscopy, nanocells offer a new tool to evaluate collisional shift and broadening, yielding an access to the open problem of collisions under confinement. It also allows probing of the atom-surface interaction in a range of unusual short distances. The experimental exploration of the distance dependence, normally evolving according to the z-3 van der Waals (vW) dependence (z : the atom-surface distance), is worth doing because it could be affected by imperfections of the real surface, such as roughness, adsorbed impurities or charges. A detailed lineshape analysis is now under progress, with tight constraints imposed to the fitting by the twin information brought by simultaneous reflection and transmission spectra. Another issue is a possible resonant enhancement, susceptible to induce a repulsive vW, due to the coupling between atom excitation and a surface mode.
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