Using BBGKY hierarchies to study the effect of the local field on the rate of radiative relaxation of quantum systems in a dielectric medium

Kuznetsov, D.V.; Roerich, V.; Gladush, M. G.

doi:10.1007/s11232-011-0089-8

Cited by 13 publications

(6 citation statements)

References 14 publications

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“…We demonstrate this approach for a polycrystalline film doped with terrylene molecules [2]. We also report a significant progress in the theory of light emission enhancement due to the local field effects [3].…”

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confidence: 85%

Local and macroscopic characterization with single molecules and single quantum emitters

et al. 2018

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We introduce an experimental approach for mapping effective local values of dielectric characteristics of solid films and the analysis of the related local-field effects. The characterisation technique is based on the imaging and spectroscopy of single chromophore molecules at cryogenic temperatures. The progress in the theory of fluorescence enhancement due to the local field effects is reported.

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confidence: 85%

Local and macroscopic characterization with single molecules and single quantum emitters

et al. 2018

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“…The fact that the local-field correction factor appears in the first power in the expression for the local-field-corrected spontaneous emission rate is typical for fully microscopic approaches [60]. For instance, another microscopic model, developed by Kuznetsov et al [61,62], leads to an expression for the spontaneous emission rate where factor L enters in the first power, similar to Eq. (31).…”

Section: Microscopic Theoriesmentioning

confidence: 99%

Local-field effects in nanostructured photonic materials

Dolgaleva

Boyd

2012

Adv. Opt. Photon.

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It is well known that the optical response of a medium depends on the local field acting on an individual emitter rather than on the macroscopic average field in the medium. The local field depends very sensitively on the microcopic environment in an optical medium. It is thus possible to achieve a significant control over the local field by intermixing homogeneous materials on a nanoscale to produce composite optical materials. A combination of local-field effects and nanostructuring provides new degrees of freedom for manipulating the optical properties of photonic materials. Especially interesting opportunities open up in the nonlinear optical regime where the material response depends on the local-field correction as a power law. The goal of this review is to present a conceptual overview of the influence of local-field effects on the optical properties of photonic materials, both homogeneous and composite. We also give a summary of recent achievements in controlling the optical properties by local-field effects and nanostructuring.

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“…Besides resonant interatomic interaction the line shape of impurity centers is transformed due to interaction with the surrounding dielectric medium (see [10] - [20]). Even in the case of a transparent dielectric the internal fields of a medium cause spectral line shifts of the impurity atoms which can exceed the natural linewidth.…”

Section: Introductionmentioning

confidence: 99%

Light trapping in an ensemble of pointlike impurity centers in a Fabry-Perot cavity

Kuraptsev

Sokolov

2016

Phys. Rev. A

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We report the development of quantum microscopic theory of quasi-resonant dipole-dipole interaction in the ensembles of impurity atoms imbedded into transparent dielectric and located into Fabry-Perot cavity. On the basis of the general approach we study the simultaneous influence of the cavity and resonant dipole-dipole interaction on the shape of the line of atomic transition as well as on light trapping in dense impurity ensembles. We analyze this influence depending on the size of the ensemble, its density, as well as on r.m.s. deviation of the transition frequency shifts caused by the symmetry disturbance of the internal fields of the dielectric medium. Obtained results are compared with the case when the cavity is absent. We show that the cavity can essentially modify cooperative polyatomic effects.

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Using BBGKY hierarchies to study the effect of the local field on the rate of radiative relaxation of quantum systems in a dielectric medium

Cited by 13 publications

References 14 publications

Local and macroscopic characterization with single molecules and single quantum emitters

Local and macroscopic characterization with single molecules and single quantum emitters

Local-field effects in nanostructured photonic materials

Light trapping in an ensemble of pointlike impurity centers in a Fabry-Perot cavity

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