Unraveling Early-Stage Dynamics of Cage-to-Covalent Organic Framework Transformation at Liquid–Liquid Interface
G. Shreeraj,
Madhvi Tiwari,
Venkateshwar Rao Dugyala
et al.
Abstract:Postsynthetic linker exchange (PLE) has emerged as an emerging synthetic strategy for constructing high-quality covalent organic frameworks (COFs) from preassembled entities such as linear polymers, amorphous networks, COFs, and porous organic cages by using the principles of dynamic covalent chemistry. The PLE strategy has recently been extended at the liquid−liquid interface to fabricate highly crystalline two-dimensional (2D)-COF membranes at a faster time scale (24 h). Examining the early stages of the int… Show more
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