Abstract:We investigate the depletion of single-electron states in small molecules under the influence of very short XUV pulses. In N2, for a certain window of XUV energies around 50 eV, we observe a marked occupation inversion, i.e. a situation where depletion of the deepest bound valence electron state is much larger than for any other state. This represents a realistic mechanism which is able to cut, almost instantaneously, a hole into a deep lying state, a situation which is often assumed ad hoc in numerous theoret… Show more
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