1922
DOI: 10.1021/ja01424a008 View full text |Buy / Rent full text
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Abstract: Since our first paper1 Venkataramaiah reported3 the independent discovery of the active form of hydrogen, distinguished by its ability to reduce potassium permanganate solution rapidly at room temperature. He produced it first in the alternating current corona, but made the interesting observation that it is produced in measurable quantities when oxygen is exploded in an excess of hydrogen. Since all other methods of its preparation, including those reported below, are dependent on prolonged and intense ioniza… Show more

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“…His student Landauer wrote his PhD thesis on this subject, probably the first ever such thesis (Landauer, 1922). In another work the two Chicago chemists reviewed methods of preparation and the experimental evidence for the new gas (Wendt and Landauer, 1922). The most consistent of the chemical tests for the existence of a relatively long‐lived active hydrogen relied on the formation of hydrogen sulfide on a deposit of sulfur powder; the produced hydrogen sulfide was typically identified by its reaction with lead acetate on strips of paper.…”
Section: The Chemists and Active Hydrogenmentioning
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“…His student Landauer wrote his PhD thesis on this subject, probably the first ever such thesis (Landauer, 1922). In another work the two Chicago chemists reviewed methods of preparation and the experimental evidence for the new gas (Wendt and Landauer, 1922). The most consistent of the chemical tests for the existence of a relatively long‐lived active hydrogen relied on the formation of hydrogen sulfide on a deposit of sulfur powder; the produced hydrogen sulfide was typically identified by its reaction with lead acetate on strips of paper.…”
Section: The Chemists and Active Hydrogenmentioning
“…Several years ago a number of publications (41,42) dealt with the production of "active" hydrogen by various methods of activation, included in which were methods involving the use of catalytic agents, notably platinum. In many of these cases claims for the production of active hydrogen were made under circumstances which seemed to violate the laws of thermodynamics.…”
Section: Surface Effects In Chain Reactionsmentioning