The current spaceborne synthetic aperture radar (SAR) systems are operated to illuminate the scene along the satellite flying direction. However, in many cases, the interested areas are not parallel to the flying direction, so an innovative smart imaging mode is acquired, which can be employed for illuminating scene along a given direction. In this paper, a novel three-axis attitude steering method is proposed for smart imaging mode. First, mathematical model of the attitude steering is built by considering the restrictive conditions of zero Doppler centroid requirement and the position of interested area. Then, an iterative optimization algorithm is designed to calculate the three-axis steering angles. Finally, experiment results using the satellite tool kit (STK) tool validate the proposed methods well, especially in the case of coastline imaging.Introduction: State-of-the-art spaceborne SAR systems have the capability of operating in different imaging modes, such as stripmap, ScanSAR, spotlight, Terrain Observation by Progressive Scans (TOPS), and sliding spotlight [1][2]. However, all of the imaging modes illuminate the scene along the satellite flying direction. It means that if the interested area is not along the flying direction, more SAR observations from different satellite orbits at different times are required, which will take a long time to cover the interested area. The ScanSAR or TOPS mode can be employed to mitigate this problem by enlarging the range-swath coverage, but at the cost of resolution [3]. Therefore, the smart imaging mode is required, which can be employed for illuminating the scene along a given direction by implementing threeaxis attitude steering. In current spaceborne SAR systems, the main purpose of attitude steering is to minimize the Doppler centroid frequency, such as the one-axis (yaw) steering method with the circular orbit assumption [4], and the two-axis (yaw and pitch) steering method by taking the eccentricity into consideration [5]. In this letter, a novel attitude steering method is proposed for the smart imaging mode with three-axis (yaw, pitch and roll) steering. The mathematical model of attitude steering is first derived by considering the restrictive conditions of zero Doppler centroid requirement and the position of interested area, followed by the optimization algorithm for three-axis steering; finally, experiments are performed to validate the proposed method.