diffraction (XRD). [6] Computationally, continuum mechanics, [7] molecular dynamics simulations, [8] and density functional theory (DFT) [9] are powerful techniques to simulate the strain conditions. The inelastic strain is generally associated with dislocation plasticity or fracture. The dislocation plasticity should be avoided in elastic strain studies since the lattice dislocation can release the elastic strain besides disturbing the original electronic structure of materials. [10] Hence, the strain in this review is limited to elastic strain unless by a particular statement. The strain effect is based on the difference in reactivity according to the atomic arrangement (involving compressed or expanded arrangements) of surface atoms. [1a] The long-range strain effect (usually includes 1-6 monolayers) differs from the ligand effect and ensemble effect (both dominate at 1-2 monolayers), impacting the surface reactivities in more than a few atomic layers. [1a,11] With the development of nanotechnologies and characterization techniques, strain effect on materials can be well engineered, tuned, and controlled toward various applications (denoted as strain engineering), such as photo-/electrocatalysis, [12] superconductivity, [13] and semiconductor devices. [14] Photocatalysis, one of the most important and promising forms of catalysis, has attracted widespread attention as an appealing and promising solution to alleviate global energy and environmental issues, while its practical application primarily remains hampered by the low η abs , η cs , and η cs (η abs : light absorption efficiency, η cs : carrier separation efficiency, η cat : catalytic efficiency). [15] These three fundamental processes govern the overall photocatalytic performance (η = η abs × η cs × η cat ). [16] A variety of modification strategies are proposed to improve the photocatalytic properties of materials (e.g., strain engineering, interface engineering, crystal facet engineering, and surface modification). [17] Amongst these modification strategies that have been investigated to date, strain engineering is allowed to precisely tune the band structure [10b,18] and carrier mobility of semiconductor photocatalysts, [19] and the adsorption energy of reaction substrates or intermediates, [9,12i,20] so it has great potential to break the bottleneck of photocatalysis. While some progress has been made regarding strained photo catalysis, many difficulties and challenges still need to be overcome, including tunable creation and measurement of strain, strained photocatalysis principles, and its further applications in various photocatalytic reactions. [20,21] In addition, strain engineering in nanomaterials applied for electrocatalysis and solar cells is likely to provide novel insights for developing high-performance Whilst the photocatalytic technique is considered to be one of the most significant routes to address the energy crisis and global environmental challenges, the solar-to-chemical conversion efficiency is still far from satisfying prac...