The right shoe for the job

Gandavadi, Dhanush; Hariadi, Rizal F.

doi:10.1126/science.abn9659

Science

2022

DOI: 10.1126/science.abn9659

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The right shoe for the job

Dhanush Gandavadi

Rizal F. Hariadi

Abstract: Natural dynein protein motors are reengineered to walk on specific artificial DNA tracks

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“…The amide structural core is ubiquitous in the fields of peptide and medicinal chemistry . Thus, efficient formation of substituted amides has gained continuous interest of synthetic chemists.…”

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confidence: 99%

Photoredox/Iron Dual-Catalyzed Insertion of Acyl Nitrenes into C–H Bonds

et al. 2022

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In this work, the use of N-acyloxybenzamides as efficient acyl nitrene precursors under photoredox/iron dual catalysis is reported. The resulting acyl nitrenes could be captured by various types of C–H bonds and S- or P-containing molecules. Mechanism investigations suggested that the formation of the acyl nitrene from the N-acyloxybenzamide occurs by a photoredox process, and it is believed that in this redox process oxidative N–H bond cleavage of the N-acyloxybenzamide occurs prior to reductive N–O bond cleavage of the N-acyloxybenzamide.

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confidence: 99%

Photoredox/Iron Dual-Catalyzed Insertion of Acyl Nitrenes into C–H Bonds

et al. 2022

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The right shoe for the job

Abstract: Natural dynein protein motors are reengineered to walk on specific artificial DNA tracks

Cited by 1 publication

References 12 publications

Photoredox/Iron Dual-Catalyzed Insertion of Acyl Nitrenes into C–H Bonds

Photoredox/Iron Dual-Catalyzed Insertion of Acyl Nitrenes into C–H Bonds

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