The Hydrogen Evolution Reaction: Using Molecular Design in Transition Metal Complexes to Control Catalytic Microenvironments on Electrode Surfaces
Logan Trowbridge,
Peter E. Sues
Abstract:Hydrogen gas and its production from renewable power sources will be an important part of decreasing global reliance on fossil fuels and developing a sustainable energy economy. Efficient electrocatalysis, however, relies on the delivery of both protons and electrons; ideally in a concerted fashion to avoid high energy intermediates, prevent charge build‐up, and circumvent large kinetic barriers. While this can be achieved using ligand design in homogenous molecular transition metal catalysts (specifically inc… Show more
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