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Cited by 101 publications
(89 citation statements)
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References 30 publications
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“…arene, 0.001 equiv. catalyst, 5 mL CF 3 COOH/1,2-dichloroethane (4:1), approximate reagent concentration 2.1 , 80°C, 5 h] a double M-X/CF 3 COO-H exchange occurs, as predicted on the basis of DFT calculations by Strassner et al [15] …”
Section: Resultsmentioning
confidence: 71%
“…arene, 0.001 equiv. catalyst, 5 mL CF 3 COOH/1,2-dichloroethane (4:1), approximate reagent concentration 2.1 , 80°C, 5 h] a double M-X/CF 3 COO-H exchange occurs, as predicted on the basis of DFT calculations by Strassner et al [15] …”
Section: Resultsmentioning
confidence: 71%
“…Remarkably, DFT calculations, performed by Strassner et al, have predicted that replacement of the two halides by trifluoroacetate anions takes place at high temperatures, like in our reaction conditions, and that the binding energy difference between the various halides and the metal is not large enough to produce effects on the kinetic outcome of the reaction. [23] On the other hand, the nature of the dicarbene ligand has an effect on catalytic activity. This effect can be appreciated by comparing the performance of a series of complexes with the same anionic ligand but different dicarbene ligands (3 and 6-9).…”
Section: Resultsmentioning
confidence: 99%
“…The catalytic conversions are within experimental error identical to the results of the bromide complex 20. This indicates that the dissociation of a counterion is a necessary condition for the activity of the complex [59].…”
Section: Alkane Oxidationmentioning
confidence: 93%
“…We found Pd(OAc) 2 [54][55][56] and Pt(acac) 2 [57] especially useful in that regard. In cases where no basic metal precursor is available it is often successful to add NaOAc as an external base [58,59].…”
Section: Scheme 4 Pathways For the Synthesis Of Nhc Metal Complexesmentioning
confidence: 99%
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