Terahertz electric field induced melting and transport of monolayer water confined in double-walled carbon nanotubes

Wu, Yue; Wang, Zi; Li, Shuang; Su, Jiaye

doi:10.1039/d4cp00007b

Phys. Chem. Chem. Phys.

2024

DOI: 10.1039/d4cp00007b

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Terahertz electric field induced melting and transport of monolayer water confined in double-walled carbon nanotubes

Yue Wu,

Zi Wang,

Shuang Li

et al.

Abstract: Monolayer ice confined in double-walled carbon nanotubes can be effectively melted using terahertz electric fields.

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Selective mass transport mediated by two-dimensional confined water: A comprehensive review

Jin,

Chen,

Liu

et al. 2024

FlatChem

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Selective mass transport mediated by two-dimensional confined water: A comprehensive review

Jin,

Chen,

Liu

et al. 2024

FlatChem

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Characterizing the Orderliness of Interfacial Water through Stretching Vibrations

Zhu,

Zhou,

et al. 2024

J. Phys. Chem. Lett.

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Spatial orderliness, which is the orderly structure of molecules, differs significantly between interfacial water and bulk water. Understanding this property is essential for various applications in both natural and engineered environments. However, the subnanometer thickness of interfacial water presents challenges for direct and rapid characterization of its structural orderliness. Herein, through molecular dynamics simulations and infrared spectral analysis of interfacial water in a graphene slit pore, we reveal a hyperbolic tangent relationship between the water ordering and its O−H stretching information in the infrared spectrum. Specifically, O−H symmetric stretching dominated in the highly ordered water structure, while a transition to the asymmetric stretching corresponded to an increase in the degree of disorder. Thus, the O−H stretching behavior could serve as a useful and quick assessment of the orderliness of interfacial water. This work provided insights into interfacial water's unique molecular network and structural dynamics and identified the stretching vibrations' key role in its degree of order, providing insight for fields such as nanotechnology, biology, and material science.

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Terahertz electric field induced melting and transport of monolayer water confined in double-walled carbon nanotubes

Abstract: Monolayer ice confined in double-walled carbon nanotubes can be effectively melted using terahertz electric fields.

Cited by 2 publications

References 40 publications

Selective mass transport mediated by two-dimensional confined water: A comprehensive review

Selective mass transport mediated by two-dimensional confined water: A comprehensive review

Characterizing the Orderliness of Interfacial Water through Stretching Vibrations

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