volume 60, issue 3, P1026-1035 1974
DOI: 10.1063/1.1681110
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Roy A. Lucht,
Terrill A. Cool

Abstract: The laser excited fluorescence method has been employed to determine rate constants for V -+ V, R and V -+ R, T relaxation HF(v = I) and DF(v = I) by CO 2 over the temperature range from 295 to 670°K. The self-deactivation rates for HF(v = I) and DF(v = I) by ground state molecules and the rate of V -+ V, R transfer from HF(~' = I) and DF(v = I) to the CO 2 (00 0 I) state exhibit a marked decrease with increasing temperature. The results provide additional evidence for the conversion of the large vibrational …

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