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Cited by 38 publications
(5 citation statements)
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“…This difference can be attributed to the oxygen-induced crosslinking of aromatic clusters obtained through low-temperature annealing, which turns into structures with a substantially higher degree of conjugation and stacking between aromatic sheets. 65 The understanding of the functionality of each component of HCMs provides guidelines to tune the morphology and conductivity of as-annealed products by optimizing the composition of the heterogeneous mixtures of HCM feedstocks and laser processing parameters.…”
Section: Toolbox Of Heavy Carbonaceous Materials (Hcm)mentioning
confidence: 99%
“…This difference can be attributed to the oxygen-induced crosslinking of aromatic clusters obtained through low-temperature annealing, which turns into structures with a substantially higher degree of conjugation and stacking between aromatic sheets. 65 The understanding of the functionality of each component of HCMs provides guidelines to tune the morphology and conductivity of as-annealed products by optimizing the composition of the heterogeneous mixtures of HCM feedstocks and laser processing parameters.…”
Section: Toolbox Of Heavy Carbonaceous Materials (Hcm)mentioning
confidence: 99%
“…These showed that the air-blowing method can effectively increase the oxygen content of pitch precursors, and the oxygen content of pitch precursors could be controlled by altering the air-blowing temperature. The main mechanism during the air-blowing process could be the oxidation of both Ar-Ar structure (biphenyl structure) generated by the decomposition of naphthenic structures and the alkyl side chains which leads to the formation of oxygen groups [24]. Therefore, it can be inferred that some oxygen functional groups (hydroxyl, carbonyl, carboxyl) could form during the controlled oxidative treatment.…”
Section: General Properties and Structural Characterization Of Pitch mentioning
confidence: 99%
“…23,26 On the one hand, the aliphatic chains are considered to be the active sites in the pre-oxidation process, because the oxygen preferentially attacks the C–H at the α-carbon atoms of aromatic molecules to form radicals, further transforming into an oxygen-containing cross-linking structure for stabilization. 27 On the other hand, the oxidative stabilization degree is determined by the diffusion rate of oxygen, which may be the rate-determining step, especially in the cases of pitches with low softening points or a large stabilization depth. 26,28…”
Section: Introductionmentioning
confidence: 99%
“…23,26 On the one hand, the aliphatic chains are considered to be the active sites in the pre-oxidation process, because the oxygen preferentially attacks the C-H at the a-carbon atoms of aromatic molecules to form radicals, further transforming into an oxygen-containing cross-linking structure for stabilization. 27 On the other hand, the oxidative stabilization degree is determined by the diffusion rate of oxygen, which may be the ratedetermining step, especially in the cases of pitches with low soening points or a large stabilization depth. 26,28 Except for the inuences of the pre-oxidation temperature, the duration time, and the category of the oxygen-containing groups on the performance in SIBs, the current investigations into the synthesis process of pitch-based HCs are far from sufficient because the literature shows the studies of these factors are restricted by the diversity of pitches.…”
Section: Introductionmentioning
confidence: 99%