a b s t r a c tWe report on the structure of C 2 H 4 /N 2 /O 2 counterflow diffusion flames at pressures up to 2.5 MPa. The concentrations of major species, aliphatics up to decane and aromatics up to indene are measured by GC-MS analysis of samples collected along the flame centerline with a capillary probe. The data are compared with results of a computational model with detailed chemistry and transport. A first set of measurements (Series 1) is performed for a fixed stoichiometric mixture fraction Z st = 0…
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