2015
DOI: 10.1103/physrevb.91.041404
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Probing of valley polarization in graphene via optical second-harmonic generation

Abstract: Valley polarization in graphene breaks inversion symmetry and therefore leads to second-harmonic generation. We present a complete theory of this effect within a single-particle approximation. It is shown that this may be a sensitive tool to measure the valley polarization created, e.g., by polarized light and, thus, can be used for a development of ultrafast valleytronics in graphene.

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Cited by 48 publications
(42 citation statements)
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References 26 publications
(38 reference statements)
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“…These effects were established to be responsible for photoconductivity, high-harmonic generation, and electron photon drag. A similar scenario can be observed in graphene: Indeed, high-harmonic generation [24][25][26], frequency mixing [27], the coherent photogalvanic effect [28], photothermoelectric effects [29,30], electron photon drag [31], the photogalvanic effect [32,33], and valley polarization [34,35] are among them.…”
Section: Theoretical Modelsupporting
confidence: 56%
“…These effects were established to be responsible for photoconductivity, high-harmonic generation, and electron photon drag. A similar scenario can be observed in graphene: Indeed, high-harmonic generation [24][25][26], frequency mixing [27], the coherent photogalvanic effect [28], photothermoelectric effects [29,30], electron photon drag [31], the photogalvanic effect [32,33], and valley polarization [34,35] are among them.…”
Section: Theoretical Modelsupporting
confidence: 56%
“…, which explicitly connects the behavior of the SHG spectrum at double-and single frequencies of the applied light. It is also worth mentioning that the contribution of the Π (2) d αβγ (ω) diagram is missing in [7].…”
Section: Shg Response From Massive Graphenementioning
confidence: 99%
“…A non-zero result for the triangular diagram can be obtained introducing a valley polarization that generates an imbalance between the two valleys, as discussed in Ref. 7.…”
Section: Shg Response From Massive Graphenementioning
confidence: 99%
“…It attracted a great deal of attention in the investigation of the use of graphene in the valleytronics. Different ways of generating a valley polarized current in graphene were proposed, such as with electromagnetic fields [15,16,17,18], trigonal warping [19,20], line defects [21,22,23], lattice strain [24,25,26,27,28,29,30,31] and also optical fields [32,33]. More recently in 2014, the first experimental observation of a valley current in graphene was performed [34].…”
Section: Introductionmentioning
confidence: 99%