2020
DOI: 10.1002/anie.202010306
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Abstract: Rapid and selective removal of micropollutants from water is important for the reuse of water resources. Despite hollow frameworks with specific functionalized porous walls for the selective adsorption based on a series of interactions, tailoring a stable shape of nanometer-and micrometer-sized architectures for the removal of specific pollutants remains a challenge. Here, exactly controlled sheets, tubes, and spherical frameworks were presented from the crosslinking of supramolecular colloids in polar solvent… Show more

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Cited by 12 publications
(13 citation statements)
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References 46 publications
(56 reference statements)
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“…The different aspects in the 3D assembly structures may be attributed to discrepancies in the solvation of an imidazolium chloride group in CH 3 CN and NMP. 60 The ionic IMCOF may be more solvated in polar NMP than in CH 3 CN, resulting in its planar 3D assembly. High-resolution TEM images and fast Fourier transform (FFT) patterns suggest that IMCOFs exhibit low crystallinity, which can facilitate ion mobility and mass transport at the solid−liquid interfaces of Zn−air batteries.…”
Section: ■ Results and Discussionmentioning
confidence: 99%
“…The different aspects in the 3D assembly structures may be attributed to discrepancies in the solvation of an imidazolium chloride group in CH 3 CN and NMP. 60 The ionic IMCOF may be more solvated in polar NMP than in CH 3 CN, resulting in its planar 3D assembly. High-resolution TEM images and fast Fourier transform (FFT) patterns suggest that IMCOFs exhibit low crystallinity, which can facilitate ion mobility and mass transport at the solid−liquid interfaces of Zn−air batteries.…”
Section: ■ Results and Discussionmentioning
confidence: 99%
“…Different solvent-polymer interactions or compatibility exert a notable inuence on the nucleation, growth, and assembly of the polymeric intermediates, thus affecting the microstructure properties of the resultant carbons. [36][37][38][39] Therefore, unraveling the role of solvent-precursor interaction to synthesize heteroatomic porous carbons with optimized microstructures would substantially promote carbon design for energy-related applications.…”
Section: Introductionmentioning
confidence: 99%
“…Covalent organic frameworks (COFs) make up an emerging class of two-dimensional (2D) and three-dimensional (3D) crystalline porous polymers, with an exceptional diversity of types and shapes, due to the high accessibility and diversity of organic building blocks. Meanwhile, these materials usually exhibit low densities, large specific surface areas, high thermal stabilities, and controllable structures, rendering them good candidates for various potential applications, including gas adsorption, organic catalysis, photocatalysis, electrochemistry, molecular recognition, fluorescence sensing, etc. COFs are constructed typically by interconnecting the molecular building blocks; therefore, the reversibility of the condensation reactions for the synthesis of highly crystalline COFs is particularly critical, while the formation of strong covalent bonds often leads to poor crystallinity or even an amorphous network.…”
Section: Introductionmentioning
confidence: 99%