2002
DOI: 10.1103/physrevb.65.073306
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Parametric pumping at finite frequency

Abstract: We report on a first principles theory for analyzing the parametric electron pump at a finite frequency. The pump is controlled by two pumping parameters with phase difference φ. In the zero frequency limit, our theory predicts the well known result that the pumped current is proportional to sin φ. For the more general situation of a finite frequency, our theory predicts a non-vanishing pumped current even when the two driving forces are in phase, in agreement with the recent experimental results. We present t… Show more

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Cited by 156 publications
(206 citation statements)
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“…Not only can this verify the validity of Marcus theory, it can also reveal some of the microscopic mechanisms of the charge transfer, e.g., the possible role of surface intermediate states, the relative importance of the electronic coupling constant versus the driving force and reorganization energy, and whether the system is in the normal or inverted Marcus region. Herein we apply a charge patching method 28 to compute charge transfer rates between a CdSe/CdS quantum rod and a surface tethered ferrocene derivative. To overcome the error associated with conventional density functional theory (DFT) in determining the band gap and orbital levels, we apply the many body perturbation GW method.…”
Section: ■ Introductionmentioning
confidence: 99%
“…Not only can this verify the validity of Marcus theory, it can also reveal some of the microscopic mechanisms of the charge transfer, e.g., the possible role of surface intermediate states, the relative importance of the electronic coupling constant versus the driving force and reorganization energy, and whether the system is in the normal or inverted Marcus region. Herein we apply a charge patching method 28 to compute charge transfer rates between a CdSe/CdS quantum rod and a surface tethered ferrocene derivative. To overcome the error associated with conventional density functional theory (DFT) in determining the band gap and orbital levels, we apply the many body perturbation GW method.…”
Section: ■ Introductionmentioning
confidence: 99%
“…The approach we take to tackle the problem of the electronic structure of conjugated polymers is centered around our recently developed charge patching method [12][13][14][15] for electronic structure of organic systems 16 which enables studies of systems with more than ten thousand atoms with the accuracy similar to the one of DFT in local density approximation (LDA). Atomic structure is found from a classical molecular dynamics (MD) simulation.…”
Section: Introductionmentioning
confidence: 99%
“…In and around a vortex core in Bi 2 Sr 2 CaCu 2 O 8+δ (BSCCO), p ∼ 4.3 1 ; p ∼ 4 in optimally doped BSCCO in zero magnetic field 2 ; p ≃ 4.7 in underdoped BSCCO in the pseudogap phase above T c 3 ; p ≃ 4 in lightly doped oxychlorides Ca 2−x Na x CuO 2 Cl 2 (Na-CCOC) at very low temperatures 4 ; and in substantially underdoped BSCCO, p ∼ 4.5 were observed in the dark regions of the conductance map 5 . The nature and the origin of the LDOS modulations, in particular the short coherence length and the role of dopants 6,7 , are unclear at present. Several inhomogeneous electronic states have been proposed theoretically, including pair density waves 8,9 ; hole Wigner crystal 10 ; a Wigner crystal of hole pairs embedded in a d-wave resonating valence bond (RVB) state 11 ; and valence-bond solid with or without charge order 12 .…”
mentioning
confidence: 99%
“…In essence, the local doping concentration x i is promoted to a variational parameter 6 . Second, as an electron hops between sites, the renormalized bandwidth will change by O(1/N s ).…”
mentioning
confidence: 99%