Abstract:The desirable self‐assembly (SA) of repeated 2D stacked layers requires a “holistic analysis” of three interconnected components: the electrode, the interface, and the molecular component; among them, the contact interface bears the largest burden responsibilities. Epitaxial growth (EG) of coherent 2D+n stacked heterojunction by solvent‐free deposition holds great promise, although the feasibility has never been demonstrated given multiple drawbacks (e.g., surface‐ligand effect, SLE). Here, it is demonstrated … Show more
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