On the origin of initial hydrocarbons in methanol-to-hydrocarbons reaction
Javier Ruiz-Martinez,
Teng Li,
Sang-Ho Chung
et al.
Abstract:Providing a complete scheme to describe the methanol-to-hydrocarbons (MTH) reaction network is impeded by insufficient understanding of the chemistry occurring incipiently. Using a temperature-dependent reaction strategy, combined with operando photoelectron photoion coincidence (PEPICO) spectroscopic diagnosis of intermediate species and theory, we provide a comprehensive understanding on initial hydrocarbons formation, including the first C–C bond, olefins, and aromatics. Surface acetyl groups attached to ze… Show more
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