but these studies have largely failed to account for realistic, experimental considerations by using pulse energies and durations that would lead to ionization of the gas (optical breakdown) or, as a result of the Fourier transform limit, would make achieving the narrowband, monochromatic nature of the interaction required for optimal heating difficult. Given these realistic experimental limitations, combined with low intrinsic energy deposition efficiency (10 −5 ), such ~2000 K temperatures changes are not likely to be realized using a traditional monochromatic singleshot implementation [12]. In an effort to sidestep this intrinsic energy deposition inefficiency, some groups have looked at heating in the context of multipass, non-resonant, optical cavities [13,14]. In these cavity configurations, a laser pulse that remains largely unaffected in the single-pass case is given increased opportunity for energy deposition, and thus higher final temperatures, over the single-pass case. While these numerical studies have predicted several fold increases in available gas temperature changes [12,13,15], the use of multipass cavities places significant experimental constraints on efforts to achieve maximum energy deposition, with optical energy losses, damage thresholds, alignment challenges, and fixed optical lattice velocities further limiting gas heating potential. Incorporating the recent development of a chirped laser for optical Stark deceleration [16], this study employs the direct simulation Monte Carlo code SMILE in an effort to provide insight into how optical lattice laser pulse parameters affect heating magnitudes attainable through optical lattice gas heating [5]. Using pulse intensities that avoid ionization of the gas [17], this work specifically looks at intrapulse frequency chirping, first proposed by Barker et al. [2], as a way to continually update lattice velocities to better reflect that required by the instantaneous state of the gas for optimal energy deposition.Abstract Direct simulation Monte Carlo was used to investigate the interaction between molecular nitrogen, argon, and methane, initially at 300 K and 0.8 atm, and frequency-chirped, pulsed optical lattices. The simulated optical lattice parameters are consistent with published optical lattice-based experiments to ensure that pulse energies and durations do not exceed optical breakdown (ionization) thresholds. In an effort to maximize optical lattice gas heating, laser pulses were chirped to produce lattice velocities which more effectively facilitate energy deposition throughout the pulse duration. The maximum end pulse translational temperature obtained in nitrogen, argon, and methane was 763, 715, and 1018 K, respectively.