“…The matrices for wound dressing applications were dominated by synthetic polymers because they were mostly used for external treatment. However, for drug delivery, antibacterial, and antioxidant applications that involve oral supplementation, natural biopolymers such as starch [146][147][148], chitosan [149][150][151], pullulan [152][153][154][155], and gelatin [156][157][158] are preferred. Polymers with good mechanical properties and flexibility, such as PCL/ PU [50][51][52], gelatin/citric acid [159], and chitosan [160][161][162] were applied for medical implant and tissue engineering applications.…”