Search citation statements
Paper Sections
Citation Types
Year Published
Publication Types
Relationship
Authors
Journals
This review provides a brief introduction to the physics of coupled exciton-plasmon systems, the theoretical description and experimental manifestation of such phenomena, followed by an account of the state-of-the-art methodology for the numerical simulations of such phenomena and supplemented by a number of FORTRAN codes, by which the interested reader can introduce himself/herself to the practice of such simulations. Applications to CW light scattering as well as transient response and relaxation are described. Particular attention is given to so-called strong coupling limit, where the hybrid exciton-plasmon nature of the system response is strongly expressed. While traditional descriptions of such phenomena usually rely on analysis of the electromagnetic response of inhomogeneous dielectric environments that individually support plasmon and exciton excitations, here we explore also the consequences of a more detailed description of the molecular environment in terms of its quantum density matrix (applied in a mean field approximation level). Such a description makes it possible to account for characteristics that cannot be described by the dielectric response model: the effects of dephasing on the molecular response on one hand, and nonlinear response on the other. It also highlights the still missing important ingredients in the numerical approach, in particular its limitation to a classical description of the radiation field and its reliance on a mean field description of the many-body molecular system. We end our review with an outlook to the near future, where these limitations will be addressed and new novel applications of the numerical approach will be pursued.
The widely-used Jones and Mueller differential polarization calculi allow non-depolarizing deterministic polarization interactions, known to be elements of the SO + (1, 3) Lorentz group, to be described in an efficient way. In this Letter, a stochastic differential Jones formalism is shown to provide a clear physical insight on light depolarization, which arises from the interaction of polarized light with a random medium showing fluctuating anisotropic properties. Based on this formalism, several intrinsic depolarization metrics naturally arise to efficiently characterize light depolarization in a medium, and an irreversibility property of depolarizing transformations is finally established.PACS numbers: 42.25.Ja; 42.25.Bs; 78.20.Bh; 89.70.Cf; 02.20.Sv In the field of polarimetry, Jones and Stokes/Mueller formalisms have always appeared as dual and often exclusive approaches, whose specific characteristics have been exploited for diverse applications. On the one hand, the description of field coherence in the Jones calculus, which relates the input and output 2-dimensional complex electric field through E out = JE in , justifies its use in ellipsometry [1,2], optical design [3-6], spectroscopy [6], astronomy [7] or radar (PolSar) [8]. On the other hand, Mueller calculus is widely used in biophotonics [9,10], material characterization [11,12] or teledetection [13], as it is based on optical field observables (intensity measurements), relating the input and output 4-dimensional real Stokes vector through s out = Ms in . As a consequence, these approaches fundamentally differ in their capacity to characterize depolarizing light-matter interactions (i.e., non-deterministic polarization transformations yielding a partial randomization of the input electric field). As Jones already pointed out in one of his seminal papers [14], Jones matrices are unable to directly describe depolarizing media, which can however be grasped in the Mueller formalism via depolarizing Mueller matrices. This discrepancy between both standpoints takes part in the debate, still topical in the scientific community, about the physical origin of light depolarization in media [15][16][17][18][19][20][21][22][23]. In this Letter, we show that the differential polarization formalism, which naturally arises from group theory, provides new physical insight on depolarizing light-matter interactions. This approach allows us to define intrinsic depolarization metrics, and to demonstrate an irreversibility property for depolarizing transformations, as a counterpart to the well-known invariance property verified by deterministic interactions.In the specific situation of a deterministic polarization transformation, there is a clear one-to-one relationship (recalled in Fig. 1) between a 2 × 2 complex Jones matrix J and the corresponding 4 × 4 real-valued nondepolarizing Mueller-Jones matrix M nd [24,25]. Interestingly, when one considers normalized unit-determinant matrices, both descriptions appear to be isomorphic representations of the same 6-dimensi...
scite is a Brooklyn-based organization that helps researchers better discover and understand research articles through Smart Citations–citations that display the context of the citation and describe whether the article provides supporting or contrasting evidence. scite is used by students and researchers from around the world and is funded in part by the National Science Foundation and the National Institute on Drug Abuse of the National Institutes of Health.
hi@scite.ai
10624 S. Eastern Ave., Ste. A-614
Henderson, NV 89052, USA
Copyright © 2024 scite LLC. All rights reserved.
Made with 💙 for researchers
Part of the Research Solutions Family.