Stretchable strain sensors have gained increasing popularity
as
wearable devices to convert mechanical deformation of the human body
into electrical signals. Two-dimensional transition metal carbides
(Ti3C2T
x
MXene)
are promising candidates to achieve excellent sensitivity. However,
MXene films have been limited in operating strain ranges due to rapid
crack propagation during stretching. In this regard, this study reports
MXene/carbon nanotube bilayer films with tunable sensitivity and working
ranges. The device is fabricated using a scalable process involving
spray deposition of well-dispersed nanomaterial inks. The bilayer
sensor’s high sensitivity is attributed to the cracks that
form in the MXene film, while the compliant carbon nanotube layer
extends the working range by maintaining conductive pathways. Moreover,
the response of the sensor is easily controlled by tuning the MXene
loading, achieving a gauge factor of 9039 within 15% strain at 1.92
mg/cm2 and a gauge factor of 1443 within 108% strain at
0.55 mg/cm2. These tailored properties can precisely match
the operation requirements during the wearable application, providing
accurate monitoring of various body movements and physiological activities.
Additionally, a smart glove with multiple integrated strain sensors
is demonstrated as a human–machine interface for the real-time
recognition of hand gestures based on a machine-learning algorithm.
The design strategy presented here provides a convenient avenue to
modulate strain sensors for targeted applications.