(Ca0.2Sr0.8)3(ZrxTi1-x)2O7 (x = 0.02-0.1) ceramic prepared by the solid state method was investigated for its microstructure and microwave dielectric properties. The correlation between the microstructure and microwave dielectric properties was also investigated. By increasing x from 0.01 to 0.06, the dielectric constant and Q×f value of the specimen could be increased from 72 to a maximum of 74, and from 11000 GHz to a maximum of 18000 GHz, respectively. The εr value of 74, the Q×f value of 18,000 GHz, and the τf value of 418 ppm/oC were obtained for (Ca0.2Sr0.8)3(Zr0.06Ti0.94)2O7 ceramics sintering at 1520oC for 4h, and (Ca0.2Sr0.8)3(ZrxTi1-x)2O7 (x = 0.02-0.1) is proposed as a suitable material candidate for application in microwave ceramic temperature sensing antenna.