We report a study of the triangular-lattice Heisenberg magnet NiGa 2 S 4 by the positive muon spin relaxation technique. We unravel three temperature regimes: ͑i͒ below T c = 9.2͑2͒ K, a spontaneous static magnetic field at the muon site is observed and the spin dynamics is appreciable: the time scale of the modes we probe is Ӎ7 ns; ͑ii͒ an unconventional stretched exponential relaxation function is found for T c Ͻ T Ͻ T cross , where T cross = 12.6 K, which is a signature of a multichannel relaxation for this temperature range; and ͑iii͒ above T cross , the relaxation is exponential as expected for a conventional compound. The transition at T c is of the continuous type. It occurs at a temperature slightly smaller than the temperature at which the specific heat displays a maximum at low temperature. This is reminiscent of the behavior expected for the BerezinskiiKosterlitz-Thouless transition. We argue that these results reflect the presence of topological defects above T c .On cooling, in the same way as liquids, magnetic materials usually crystallize to form long-range periodic arrays. However, magnetic materials with antiferromagnetically coupled spins located on triangular motifs exhibit geometrical magnetic frustration which may prevent the crystallization to occur. 1 Such materials are a fertile ground for the emergence of novel spin-disordered states such as spin liquid or spin glass even without crystalline disorder. The simplest example of geometrical frustration, stacked two-dimensional triangular lattices with a single magnetic ion per unit cell, has been studied intensively. 2 NiGa 2 S 4 is a rare example of such a two-dimensional antiferromagnet which does not exhibit a long-range magnetic order at low temperature and which is characterized by gapless excitations. 3,4 These physical properties lead naturally to the assumption that its ground state is a spin liquid. Here, we report muon spin rotation and relaxation ͑SR͒ measurements which show that a spontaneous static magnetic field appears below T c = 9.2͑2͒ K where an appreciable spin dynamics is measured. In addition, we find the spin dynamics to be unconventional in the temperature range T c Ͻ T Ͻ T cross , where T cross = 12.6 K.Polycrystalline powder of NiGa 2 S 4 has been obtained from a solid-vapor reaction using a stoichiometric mixture of pure elements. The synthesis took place in an evacuated silica ampoule. A slow heat treatment over several days up to 1000°C has been performed with respect to the high sulfur vapor pressure. 5 After a final grinding, the powder was treated for a week at 1000°C. NiGa 2 S 4 is a chalcogenide magnetic insulator with the Ni 2+ magnetic ions ͑spin S =1͒ sitting on a regular triangular lattice. The interactions are of the Heisenberg type, referring to the isotropic Curie constant. 4 The crystal structure consists of two GaS layers and a central NiS 2 layer stacked along the c axis. A Rietveld refinement of a neutron powder diffraction pattern recorded at 50 K at the cold neutron powder diffractometer DMC of th...