“…[3][4][5][6][7][8][9] UC refers to an anti-Stokes type nonlinear optical emission process in which one higher energy photon is emitted for every two or more absorbed lower energy photons. 10 Since the first experimental demonstration in 1966, 11 this effect has received renewed interest due to its ever expanding application base in, for example, lasing, 12 laser cooling, 13 temperature sensing, 14 biomedical imaging and therapy, 15,16 3D displays, 17 and, more recently, for broadening the spectral response of PV devices. [4][5][6][7][8][9] In the context of Si PV devices, the UC of the sub-bandgap photons (k > 1100 nm) into above-bandgap photons (k < 1100 nm) increases the theoretical efficiency limit of a single-junction Si solar cell from near 30% up to 40% when illuminated under non-concentrated light.…”