2000
DOI: 10.1103/physrevlett.85.4743
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Heterogeneous Hole Nucleation in Electron-ChargedH4eWetting Films

Abstract: 4He wetting layers on Cs exhibit an unusually long-lived metastable state upon undercooling to temperatures well below the wetting temperature T(w) approximately 1.9 K. The decay of this state by homogeneous thermal nucleation of holes is disfavored by the incipient divergence of the free energy barrier separating the metastable thick film from the stable thin-film state. We propose that interface deformations ("dimples") created by electrons bound at the 4He liquid-vapor interface can be used as nuclei for th… Show more

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Cited by 4 publications
(3 citation statements)
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“…The effect of the nature of the substrate has been studied by several authors namely [4] the critical wetting of pentane on water. The critical adsorption and the layering transitions, at the free surface, of a smectic liquid crystal [5], the effect of segregation on wetting in films of a partially miscible polymer blend [6], the effect of the chain length of alkanes on water [7], the critical adsorption and dimensional crossover in epitaxial FeCo films [8], the heterogeneous hole nucleation in electron-charged 4 He wetting films [9], the existence of tricritical wetting in liquid mixtures of methanol and the n-alkanes [10]. The dynamic aspect has been studied for fluid interface of nanometric curvature formed by capillary condensation between solid substrates [11], for wetting layers [12], and for layering transition in confined liquids [13].…”
Section: Introductionmentioning
confidence: 99%
“…The effect of the nature of the substrate has been studied by several authors namely [4] the critical wetting of pentane on water. The critical adsorption and the layering transitions, at the free surface, of a smectic liquid crystal [5], the effect of segregation on wetting in films of a partially miscible polymer blend [6], the effect of the chain length of alkanes on water [7], the critical adsorption and dimensional crossover in epitaxial FeCo films [8], the heterogeneous hole nucleation in electron-charged 4 He wetting films [9], the existence of tricritical wetting in liquid mixtures of methanol and the n-alkanes [10]. The dynamic aspect has been studied for fluid interface of nanometric curvature formed by capillary condensation between solid substrates [11], for wetting layers [12], and for layering transition in confined liquids [13].…”
Section: Introductionmentioning
confidence: 99%
“…Meanwhile, in a combined effort of experimentalists and theorists, a very good quantitative understanding of these processes has been achieved [2][3][4][5]. Thin film instabilities can also be triggered by defects, such as vortices in undercooled wetting films of helium on alkali metals [6][7][8] or by the application of thermal gradients to confined polymer films [9][10][11]. For the helium films, the situation is slightly complicated due to the pronounced substrate disorder effects [12,13] which, however, are irrelevant for the strongly asymmetric thermal hysteresis that is common to all wetting systems [14,15,1].…”
Section: Introductionmentioning
confidence: 99%
“…(3.1) which has to be included with a Lagrange multiplier), but that the functional form of the surface charge density nðrÞ is fixed as well. We then only need to parametrize nðrÞ in a convenient way which lends itself to analytic calculations [94].…”
Section: The Harmonic Model and Its Approximate Solutionsmentioning
confidence: 99%