Electrocatalytic dechlorination of aqueous trichloroacetic acid by Vitamin B12 modified iron electrode

Ma, Xiaoyan; Huang, Sinong; Jin, Yuhong; Jiang, Hang; Tang, Luping; Wu, Yifei; Ni, Yajuan; Zhu, Shiqun; Li, Xueyan; Dietrich, Andrea M.

doi:10.1016/j.jece.2023.109944

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Degradation Of Pollutants By Molecular Inspired Electrocatal...1

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2023

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“…106 Cobalamin, or vitamin B12 (VB12), can be used for the dechlorination of trichloroacetic acid to produce acetic acid in a 93% at a j of −7 mA cm −2 under 5 h, with dichloroacetic acid and monochloroacetic acid as minor byproducts. 107 Similarly, VB12 can also debrominate tribromoacetic acid with 99% of FE after 6 h under optimal galvanostatic conditions ( j = −10.0 mA cm −2 ). In situ Raman spectroscopy shows Co–Br bond formation, which significantly enhances the electron transfer due to is the main step to initiate the debromination process.…”

Section: Degradation Of Pollutants By Molecular Inspired Electrocatal...mentioning

confidence: 99%