Abstract.The western tropical South Pacific was sampled along a longitudinal 4000 km transect (OUTPACE cruise, 18 Feb., 3 Apr. 2015) for measurement of carbonates parameters (total alkalinity and total inorganic carbon) between the Melanesian Archipelago (MA) and the western part of the South Pacific gyre (WGY). This manuscript reports this new dataset and derived properties: pH on the total scale (pHT) and the CaCO3 saturation state with respect to calcite (Ωcal) and aragonite (Ωara). We also estimate anthropogenic carbon (CANT) distribution in the water column using the TrOCA method (Tracer combining Oxygen, inorganic Carbon and total Alkalinity). Along the OUTPACE transect, CANT inventories of 37 -43 mol m -2 were estimated with higher CANT inventories in MA waters (due to a deeper penetration of CANT in the intermediate waters) than in the WGY waters although highest CANT concentrations were detected in the sub-surface waters of WGY. By combining our OUTPACE dataset with data available in GLODAPv2 (1974GLODAPv2 ( -2009, temporal changes in oceanic inorganic carbon were evaluated. An increase of 1.3 to 1.6 µmol kg
IntroductionHuman activities inject about 10 13 kg of carbon per year to the atmosphere which might have major consequences on climate. It is recognized that the ocean plays a key role in the control of atmospheric CO2 through uptake by the so called "oceanic carbon pump". Through this "pump", the ocean sequesters ca. 30% of the CO2 injected annually in the atmosphere by human activities (Le Quéré et al., 2018). A consequence of the ocean carbon uptake is a decrease of the oceanic pH (Feely et al, 2004) which is described as ocean acidification (the so-called "other" CO2 problem). Effects of ocean acidification have been observed on marine organisms and could affect the marine ecosystems (Riebesell et al., 2000). Improving our understanding of the oceanic CO2 uptake relies primarily on observations of the marine carbonate cycle. Studies on the oceanic carbonate cycle have been mostly conducted in the frame of international programs. The World Ocean Circulation Experiment (WOCE) and the Joint Global Flux Study (JGOFS) in the 90's have coordinated oceanographic cruises along large sections in the ocean to collect samples through the water column and to perform accurate measurements of carbonate parameters and ancillary parameters (temperature, salinity, dissolved oxygen, nutrients,...). Since 2000, efforts have been made to "revisit" oceanic sections according to the WOCE strategy in order to assess oceanic changes at the scale of a decade. These programs have generated important databases for oceanic carbonate chemistry (e.g. GLODAP_V2 -Olsen et al., 2016).In order to better assess the role of the ocean on the global carbon cycle, the concept of oceanic anthropogenic carbon (hereafter named CANT) has been introduced and refers to the fraction of dissolved inorganic carbon (CT) in the ocean that originates from carbon injected by human activities in the atmosphere since the industrial revolutio...