“…22,32,33 Carbon materials include carbon black, carbon nanotubes, graphene and their derivatives. 12,15,36,37 Among the above materials, we choose three-dimensional graphene as the support of the catalyst, which has the advantages of large specic surface area, interconnected ordered pore structure, abundant active sites, excellent electrical conductivity, lightweight and good mechanical strength comparing with other carbon materials. 22,34,35 These advantages can enhance the electron transport capacity of the electrocatalyst, increase the contact area between the catalyst and the electrolyte solution, and accelerate the release of reaction gases.…”